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Synergetic Effect of Bi2WO6 Photocatalyst with C60 and Enhanced Photoactivity under Visible Irradiation
Abstract
Fullerene (C60)-modified Bi2WO6 photocatalyst is prepared by a simple absorbing process. The as-prepared samples show the high efficiency for the degradation of nonbiodegradable azodyes methylene blue (MB) and rhodamine B (RhB) under visible light (lamda >420 nm) and simulated solar light (lamda >290 nm). After being modified by C60, the photocatalytic activities of Bi2WO6 samples increase about 5.0 and 1.5 times for the degradation of MB and RhB under visible light irradiation, whereas 4.6 and 2.1 times under xenon lamp irradiation, respectively. The enhanced photocatalytic activity for C60-modified Bi2WO6 comes from the high migration efficiency of photoinduced electrons on the interface of C60 and Bi2WO6 which is produced by the interaction of Bi2WO6 and C60 with the conjugative pi-system. The optimum synergetic effect is found at a weight ratio of 1.25 wt % (C60/Bi2WO6). The photocatalytic reaction process of C60-modified Bi2WO6 is mainly governed by direct holes and O2*- oxidation.
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Cites
Photocatalysis on TiO2 Surfaces: Principles, Mechanisms, and Selected Results
Linsebigler, A. L., Lu, G., & Yates, J. T. (1995) · Chemical Reviews · doi:10.1021/cr00035a013 · Cited by 11,575
Cited by
Tan, H. L., Amal, R., & Ng, Y. H. (2017) · Journal of Materials Chemistry A · doi:10.1039/c7ta04441k · Cited by 459
Dong, F., Guo, S., Wang, H., Li, X., & Wu, Z. (2011) · The Journal of Physical Chemistry C · doi:10.1021/jp111916q · Cited by 401
Yang, M.-Q., Zhang, N., & Xu, Y.-J. (2013) · ACS Applied Materials & Interfaces · doi:10.1021/am3029798 · Cited by 365
Arora, I., Chawla, H., Chandra, A., Sagadevan, S., & Garg, S. (2022) · Inorganic Chemistry Communications · doi:10.1016/j.inoche.2022.109700 · Cited by 291
Metadata
- Authors
- Zhu, S., Xu, T., Fu, H., Zhao, J., & Zhu, Y.
- Venue
- Environmental Science & Technology
- Publisher
- American Chemical Society (ACS)
- Published
- 2007-08-08
- Volume
- 41
- Issue
- 17
- Pages
- 6234-6239
- ISSN
- 0013-936X (ISSN-L)
- 1520-5851
- OpenAlex
- W2008429578
- Cited by
- 338
- References
- 1
- FWCI
- 7.12
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhu, S., Xu, T., Fu, H., Zhao, J., & Zhu, Y. (2007). Synergetic Effect of Bi2WO6 Photocatalyst with C60 and Enhanced Photoactivity under Visible Irradiation. Environmental Science & Technology. https://doi.org/10.1021/es070953y
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