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Photocorrosion Inhibition and Enhancement of Photocatalytic Activity for ZnO via Hybridization with C60
Abstract
C60 molecules with monomolecular layer state dispersed on the surface of ZnO and formed the hybridized interaction between ZnO and C60. C60-hybridized ZnO photocatalyst showed enhanced photocatalytic activity for the degradation of the organic dye and the photocorrosion of ZnO was successfully inhibited bythe hybridization of C60 molecules. The photocorrosion inhibition of ZnO by C60 molecule could be attributed to the reduced activation of surface oxygen atom. The enhanced photocatalytic activity for C60-hybridized ZnO was originated from the high migration efficiency of photoinduced electrons on the interface of C60 and ZnO, which was produced by the interaction of C60 and ZnO with a conjugative pi-system. The enhancement degree of photocatalytic activity was strongly depended on the coverage of C60 molecules on the surface of ZnO nanoparticles, and the optimum hybridization effect was found at a weight ratio of 1.5% (C60/ZnO). The hybridization of C60 with semiconductors could be used to improve the photocatalytic activity as well as the photostability.
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Environmental applications of semiconductor photocatalysis
Hoffmann, M. R., Martin, S. T., Choi, W., & Bahnemann, D. W. (1995) · Chemical Reviews · doi:10.1021/cr00033a004 · Cited by 18,495
Cited by
Ong, W.-J., Tan, L.-L., Ng, Y. H., Yong, S.-T., & Chai, S.-P. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00075 · Cited by 7,147
Recent developments of zinc oxide based photocatalyst in water treatment technology: A review
Lee, K. M., Lai, C. W., Ngai, K. S., & Juan, J. C. (2016) · Water Research · doi:10.1016/j.watres.2015.09.045 · Cited by 2,341
Kapilashrami, M., Zhang, Y., Liu, Y.-S., Hagfeldt, A., & Guo, J. (2014) · Chemical Reviews · doi:10.1021/cr5000893 · Cited by 508
Tan, H. L., Amal, R., & Ng, Y. H. (2017) · Journal of Materials Chemistry A · doi:10.1039/c7ta04441k · Cited by 459
Yang, M.-Q., Zhang, N., & Xu, Y.-J. (2013) · ACS Applied Materials & Interfaces · doi:10.1021/am3029798 · Cited by 365
Metadata
- Authors
- Fu, H., Xu, T., Zhu, S., & Zhu, Y.
- Venue
- Environmental Science & Technology
- Publisher
- American Chemical Society (ACS)
- Published
- 2008-10-04
- Volume
- 42
- Issue
- 21
- Pages
- 8064-8069
- ISSN
- 0013-936X (ISSN-L)
- 1520-5851
- OpenAlex
- W2037103936
- Cited by
- 507
- References
- 1
- FWCI
- 7.54
- Type
- journal article
- Language
- en
- Open access
- closed
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- Fu, H., Xu, T., Zhu, S., & Zhu, Y. (2008). Photocorrosion Inhibition and Enhancement of Photocatalytic Activity for ZnO via Hybridization with C60. Environmental Science & Technology. https://doi.org/10.1021/es801484x
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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