The DOI matches its Crossref record; 26 of the 26 references it cites were found in a registry or an index.
Oxidative Removal of Bisphenol A by Manganese Dioxide: Efficacy, Products, and Pathways
Abstract
Bisphenol A (BPA) is a ubiquitous environmental contaminant with endocrine disruption potential. In this study, exploiting the outstanding oxidative capacity of manganese dioxide (delta-MnO2), we explored forthe firsttime the efficacy and mechanisms of BPA removal by MnO2. In aqueous solutions, MnO2 demonstrated an extremely efficient capacity to remove BPA. Nearly all BPA (>99%) was eliminated in 6 min in a pH 4.5 solution initially containing 800 microM MnO2 and 4.4 microM BPA. While humic acid showed negligible inhibition on BPA removal, coexisting metal ions such as Mn2+, Ca2+, Mg2+, and Fe3+ displayed suppressive effects and the inhibitive capacityfollowed the order Mn2+ > Ca2+ > Mg2+ approximately Fe3+. A total of 11 products or intermediates were indentified and a detailed reaction scheme was suggested. The products could be ascribed to a suite of reactions of radical coupling, fragmentation, substitution, and elimination, triggered by the BPA radical formed through electron transfers to MnO2. The exceptional efficiency of MnO2 in removing BPA represents a potential use of MnO2 to treat waters containing phenolic compounds and also suggests a potentially important role of oxide-facilitated abiotic transformations in BPA attenuation in natural soil and sediment environments.
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Cites
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Bisphenol A Exposure Causes Meiotic Aneuploidy in the Female Mouse
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Reductive Dissolution of Manganese(III/Iv) Oxides by Substituted Phenols
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Cited by
Biogeochemical Redox Processes and their Impact on Contaminant Dynamics
Borch, T., Kretzschmar, R., Kappler, A., Cappellen, P. V., Ginder-Vogel, M., Voegelin, A., & Campbell, K. (2010) · Environmental Science & Technology · doi:10.1021/es9026248 · Cited by 1,456
Zhu, S., Li, X., Kang, J., Duan, X., & Wang, S. (2019) · Environmental Science & Technology · doi:10.1021/acs.est.8b04669 · Cited by 1,246
A critical review of the reactivity of manganese oxides with organic contaminants
Remucal, C. K., & Ginder-Vogel, M. (2014) · Environmental Science: Processes & Impacts · doi:10.1039/c3em00703k · Cited by 375
Fate of Bisphenol A in Terrestrial and Aquatic Environments
Im, J., & Löffler, F. E. (2016) · Environmental Science & Technology · doi:10.1021/acs.est.6b00877 · Cited by 305
Wang, L., Jiang, J., Pang, S.-Y., Zhou, Y., Li, J., Sun, S., Gao, Y., & Jiang, C. (2018) · Chemical Engineering Journal · doi:10.1016/j.cej.2018.07.103 · Cited by 293
Wang, C., Zhang, H., Li, F., & Zhu, L. (2010) · Environmental Science & Technology · doi:10.1021/es101890w · Cited by 261
Mpatani, F. M., Han, R., Aryee, A. A., Kani, A. N., Li, Z., & Qu, L. (2021) · Science of The Total Environment · doi:10.1016/j.scitotenv.2021.146629 · Cited by 182
Metadata
- Authors
- Lin, K., Liu, W., & Gan, J.
- Venue
- Environmental Science & Technology
- Publisher
- American Chemical Society (ACS)
- Published
- 2009-04-14
- Volume
- 43
- Issue
- 10
- Pages
- 3860-3864
- ISSN
- 0013-936X (ISSN-L)
- 1520-5851
- OpenAlex
- W2048628028
- Cited by
- 337
- References
- 26
- FWCI
- 8.82
- Type
- journal article
- Language
- en
- Open access
- closed
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