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Size and Composition Distribution of Fine Particulate Matter Emitted from Motor Vehicles

Kleeman, Michael J., Schauer, James J., Cass, Glen R.·2000·Environmental Science & Technology

Abstract

A dilution source sampling system is augmented to measure the size-distributed chemical composition of fine particle emissions from motor vehicles. Measurements are made using an optical particle counter (OPC), a differential mobility analyzer (DMA)/condensation nucleus counter (CNC) combination, and a pair of microorifice uniform deposit impactors (MOUDIs). The sources tested with this system include catalyst-equipped gasoline-powered light-duty vehicles, noncatalyst gasoline-powered light-duty vehicles, and medium-duty diesel trucks. Chemical composition analysis demonstrates that particles emitted from the gasoline-powered vehicles tested are largely composed of organic compounds while particles emitted from diesel engines contain roughly equal amounts of organic compounds and elemental carbon. The particle mass distributions from all mobile sources tested have a single mode that peaks at approximately 0.1−0.2 μm particle diameter. Of the two diesel vehicles tested, the vehicle with the lowest fine particle emissions rate released the largest number of ultrafine particles, a finding similar to that of Bagley et al. ( Characterization of fuel and aftertreatment device effects on diesel emissions; Technical Report 76; Health Effects Institute: Cambridge, MA, 1996). Particle size distribution measurements taken throughout the FTP urban driving cycle used to test all of the vehicles described in this paper reveal that particulate mass emission rates and particulate size distributions from the vehicles tested here are similar during the cold start and hot start segments of the driving cycle.

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Metadata

Authors
Kleeman, M. J., Schauer, J. J., & Cass, G. R.
Venue
Environmental Science & Technology
Published
2000-02-19
Volume
34
Issue
7
Pages
1132-1142
ISSN
  • 0013-936X (ISSN-L)
  • 1520-5851
OpenAlex
W2061049779
Cited by
480
References
0
FWCI
65.41
Type
journal article
Language
en
Open access
closed

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CoChat. (2026). Citation check: Size and Composition Distribution of Fine Particulate Matter Emitted from Motor Vehicles. https://app.cochat.ai/papers/10.1021/es981276y
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Kleeman, M. J., Schauer, J. J., & Cass, G. R. (2000). Size and Composition Distribution of Fine Particulate Matter Emitted from Motor Vehicles. Environmental Science & Technology. https://doi.org/10.1021/es981276y

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