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H2 Evolution and Molecular Electrocatalysts: Determination of Overpotentials and Effect of Homoconjugation
Abstract
In an effort to standardize the determination of overpotential values for H(2)-evolving catalysts in non-aqueous solvents and allow a reliable comparison of catalysts prepared and assayed by different groups, we propose to adopt the half-wave potential as reference potential. We provide a simple method for measuring it from usual stationary cyclic voltammograms, and we derive the formulas to which the measured potential should be compared, taking into account the effect of homoconjugation. We also revisit tabulated values of the standard reduction potential of protons in nonaqueous solvents, E(H+/H(2))°.
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Cites
Computational high-throughput screening of electrocatalytic materials for hydrogen evolution
Greeley, J., Jaramillo, T. F., Bonde, J., Chorkendorff, I., & Nørskov, J. K. (2006) · Nature Materials · doi:10.1038/nmat1752 · Cited by 4,097
Cited by
Electrolysis of low-grade and saline surface water
Tong, W., Forster, M., Dionigi, F., Dresp, S., Sadeghi Erami, R., Strasser, P., Cowan, A. J., & Farràs, P. (2020) · Nature Energy · doi:10.1038/s41560-020-0550-8 · Cited by 1,299
Thoi, V. S., Sun, Y., Long, J. R., & Chang, C. J. (2013) · Chem. Soc. Rev. · doi:10.1039/c2cs35272a · Cited by 668
Electrocatalytic Hydrogen Evolution in Acidic Water with Molecular Cobalt Tetraazamacrocycles
McCrory, C. C. L., Uyeda, C., & Peters, J. C. (2012) · Journal of the American Chemical Society · doi:10.1021/ja210661k · Cited by 351
Metadata
- Authors
- Fourmond, V., Jacques, P.-A., Fontecave, M., & Artero, V.
- Venue
- Inorganic Chemistry
- Publisher
- American Chemical Society (ACS)
- Published
- 2010-10-21
- Volume
- 49
- Issue
- 22
- Pages
- 10338-10347
- ISSN
- 0020-1669 (ISSN-L)
- 1520-510X
- OpenAlex
- W2328034507
- Cited by
- 492
- References
- 1
- FWCI
- 8.01
- Type
- journal article
- Language
- en
- Open access
- closed
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- Fourmond, V., Jacques, P.-A., Fontecave, M., & Artero, V. (2010). H2 Evolution and Molecular Electrocatalysts: Determination of Overpotentials and Effect of Homoconjugation. Inorganic Chemistry. https://doi.org/10.1021/ic101187v
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