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Simulation of Enthalpy and Capacity of CO2 Absorption by Aqueous Amine Systems
Abstract
A model has been developed to predict the CO 2 capacity of amine-based solvent systems as well as the enthalpy associated with absorption/desorption. This model can be used to accurately predict the behavior of well-characterized solvent systems under a range of different conditions. Alternatively, the model can be used to estimate the properties of less well-defined systems as part of an initial rapid screening procedure. Investigation into the effects of varying amine basicity and degree of carbamate formation indicates that there is considerable room for improvement on the standard MEA (monoethanolamine) system in terms of both capture capacity and enthalpy of CO 2 desorption.
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Citations
Cites
The Scientific Consensus on Climate Change
Oreskes, N. (2004) · Science · doi:10.1126/science.1103618 · Cited by 1,814
Cited by
Progress and trends in CO2 capture/separation technologies: A review
Mondal, M. K., Balsora, H. K., & Varshney, P. (2012) · Energy · doi:10.1016/j.energy.2012.08.006 · Cited by 1,019
Puxty, G., Rowland, R., Allport, A., Yang, Q., Bown, M., Burns, R., Maeder, M., & Attalla, M. (2009) · Environmental Science & Technology · doi:10.1021/es901376a · Cited by 572
Self-citationCarbon dioxide utilization with C–N bond formation: carbon dioxide capture and subsequent conversion
Yang, Z.-Z., He, L.-N., Gao, J., Liu, A.-H., & Yu, B. (2012) · Energy & Environmental Science · doi:10.1039/c2ee02774g · Cited by 520
Gutowski, K. E., & Maginn, E. J. (2008) · Journal of the American Chemical Society · doi:10.1021/ja804654b · Cited by 419
Chemically Tunable Ionic Liquids with Aprotic Heterocyclic Anion (AHA) for CO2 Capture
Seo, S., Quiroz-Guzman, M., DeSilva, M. A., Lee, T. B., Huang, Y., Goodrich, B. F., Schneider, W. F., & Brennecke, J. F. (2014) · The Journal of Physical Chemistry B · doi:10.1021/jp502279w · Cited by 265
Metadata
- Authors
- McCann, N., Maeder, M., & Attalla, M.
- Venue
- Industrial & Engineering Chemistry Research
- Publisher
- American Chemical Society (ACS)
- Published
- 2008-02-23
- Volume
- 47
- Issue
- 6
- Pages
- 2002-2009
- ISSN
- 0888-5885 (ISSN-L)
- 1520-5045
- OpenAlex
- W2003499044
- Cited by
- 174
- References
- 1
- FWCI
- 22.76
- Type
- journal article
- Language
- en
- Open access
- closed
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- McCann, N., Maeder, M., & Attalla, M. (2008). Simulation of Enthalpy and Capacity of CO2 Absorption by Aqueous Amine Systems. Industrial & Engineering Chemistry Research. https://doi.org/10.1021/ie070619a
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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