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High-Performance, Solution-Processed Organic Thin Film Transistors from a Novel Pentacene Precursor
Abstract
The Lewis acid-catalyzed Diels-Alder reaction of the organic semiconductor pentacene with N-sulfinylacetamide yields a soluble adduct. Spin-coated thin films of this adduct undergo solid-phase conversion to form thin films of pentacene at moderate temperatures. Organic thin film transistors fabricated by spin-coating this adduct, followed by thermal conversion to pentacene, exhibit the highest mobility reported to date for a solution-processed organic semiconductor.
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Citations
Cited by
The Larger Acenes: Versatile Organic Semiconductors
Anthony, J. E. (2008) · Angewandte Chemie International Edition · doi:10.1002/anie.200604045 · Cited by 2,100
Charge Carrier Transporting Molecular Materials and Their Applications in Devices
Shirota, Y., & Kageyama, H. (2007) · Chemical Reviews · doi:10.1021/cr050143+ · Cited by 1,756
Semiconductors for organic transistors
Facchetti, A. (2007) · Materials Today · doi:10.1016/s1369-7021(07)70017-2 · Cited by 874
Organic thin film transistors: From theory to real devices
Horowitz, G. (2004) · Journal of Materials Research · doi:10.1557/jmr.2004.0266 · Cited by 852
Micro- and Nanopatterning Techniques for Organic Electronic and Optoelectronic Systems
Menard, E., Meitl, M. A., Sun, Y., Park, J.-U., Shir, D. J.-L., Nam, Y.-S., Jeon, S., & Rogers, J. A. (2007) · Chemical Reviews · doi:10.1021/cr050139y · Cited by 658
Metadata
- Authors
- Afzali, A., Dimitrakopoulos, C. D., & Breen, T. L.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2002-07-01
- Volume
- 124
- Issue
- 30
- Pages
- 8812-8813
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2083833784
- Cited by
- 459
- References
- 0
- FWCI
- 30.50
- Type
- journal article
- Language
- en
- Open access
- closed
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- Afzali, A., Dimitrakopoulos, C. D., & Breen, T. L. (2002). High-Performance, Solution-Processed Organic Thin Film Transistors from a Novel Pentacene Precursor. Journal of the American Chemical Society. https://doi.org/10.1021/ja0266621
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Bibliographic data: Semantic Scholar, OpenAlex, Crossref.
Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
