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The Influence of Metal Cluster Size on Adsorption Energies: CO Adsorbed on Au Clusters Supported on TiO2
Abstract
Infrared reflection absorption spectroscopy (IRAS) has been used to study CO adsorption on Au clusters ranging in size from 1.8 to 3.1 nm, supported on TiO(2). The adsorbed CO vibrational frequency blue-shifts slightly (approximately 4 cm(-)(1)) compared to that adsorbed on bulk Au, whereas the heats of adsorption (-DeltaH(ads)) increase sharply with decreasing cluster size, from 12.5 to 18.3 kcal/mol.
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Cited by
Stabilization of Platinum Oxygen-Reduction Electrocatalysts Using Gold Clusters
Zhang, J., Sasaki, K., Sutter, E., & Adzic, R. R. (2007) · Science · doi:10.1126/science.1134569 · Cited by 1,779
Metadata
- Authors
- Meier, D. C., & Goodman, D. W.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2004-01-24
- Volume
- 126
- Issue
- 6
- Pages
- 1892-1899
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2022883606
- Cited by
- 254
- References
- 0
- FWCI
- 12.91
- Type
- journal article
- Language
- en
- Open access
- closed
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- Meier, D. C., & Goodman, D. W. (2004). The Influence of Metal Cluster Size on Adsorption Energies: CO Adsorbed on Au Clusters Supported on TiO2. Journal of the American Chemical Society. https://doi.org/10.1021/ja030359y
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Bibliographic data: Semantic Scholar, OpenAlex, Crossref.
Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
