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Highly Efficient Dye-Sensitized Solar Cells with a Titania Thin-Film Electrode Composed of a Network Structure of Single-Crystal-like TiO2 Nanowires Made by the “Oriented Attachment” Mechanism
Abstract
In this study, single-crystal-like anatase TiO(2) nanowires were formed in a network structure by surfactant-assisted self-assembling processes at low temperature. The crystal lattice planes of the nanowires and networks of such wires composed of many nanoparticles were almost perfectly aligned with each other due to the "oriented attachment" mechanism, resulting in the high rate of electron transfer through the TiO(2) nanonetwork with single-crystal-like anatase nanowires. The direction of crystal growth of oriented attachment was controlled by changing the mole ratio of acetylacetone to Ti, that is, regulating both the adsorption of surfactant molecules via control of the reaction rate and the surface energy. A single-crystalline anatase exposing mainly the [101] plane has been prepared, which adsorbed ruthenium dye over 4 times higher as compared to P-25. A high light-to-electricity conversion yield of 9.3% was achieved by applying the titania nanomaterials with network structure as the titania thin film of dye-sensitized solar cells.
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Citations
Cites
A low-cost, high-efficiency solar cell based on dye-sensitized colloidal TiO2 films
O'Regan, B., & Grätzel, M. (1991) · Nature · doi:10.1038/353737a0 · Cited by 28,599
Shape control of CdSe nanocrystals
Peng, X., Manna, L., Yang, W., Wickham, J., Scher, E., Kadavanich, A., & Alivisatos, A. P. (2000) · Nature · doi:10.1038/35003535 · Cited by 4,487
Cited by
Colloidal nanocrystal synthesis and the organic–inorganic interface
Yin, Y., & Alivisatos, A. P. (2005) · Nature · doi:10.1038/nature04165 · Cited by 3,273
Nazeeruddin, M. K., De Angelis, F., Fantacci, S., Selloni, A., Viscardi, G., Liska, P., Ito, S., Takeru, B., & Grätzel, M. (2005) · Journal of the American Chemical Society · doi:10.1021/ja052467l · Cited by 2,749
Nanotechnology‐Enabled Energy Harvesting for Self‐Powered Micro‐/Nanosystems
Wang, Z. L., & Wu, W. (2012) · Angewandte Chemie International Edition · doi:10.1002/anie.201201656 · Cited by 1,063
Advances in Liquid‐Electrolyte and Solid‐State Dye‐Sensitized Solar Cells
Snaith, H. J., & Schmidt‐Mende, L. (2007) · Advanced Materials · doi:10.1002/adma.200602903 · Cited by 616
Synthesis of M@TiO2 (M = Au, Pd, Pt) Core–Shell Nanocomposites with Tunable Photoreactivity
Zhang, N., Liu, S., Fu, X., & Xu, Y.-J. (2011) · The Journal of Physical Chemistry C · doi:10.1021/jp2009989 · Cited by 594
Metadata
- Authors
- Adachi, M., Murata, Y., Takao, J., Jiu, J., Sakamoto, M., & Wang, F.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2004-10-23
- Volume
- 126
- Issue
- 45
- Pages
- 14943-14949
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2049656104
- Cited by
- 866
- References
- 2
- FWCI
- 26.60
- Type
- journal article
- Language
- en
- Open access
- closed
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- Adachi, M., Murata, Y., Takao, J., Jiu, J., Sakamoto, M., & Wang, F. (2004). Highly Efficient Dye-Sensitized Solar Cells with a Titania Thin-Film Electrode Composed of a Network Structure of Single-Crystal-like TiO2 Nanowires Made by the “Oriented Attachment” Mechanism. Journal of the American Chemical Society. https://doi.org/10.1021/ja048068s
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