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Adsorption of Molecular Hydrogen on Coordinatively Unsaturated Ni(II) Sites in a Nanoporous Hybrid Material
Abstract
A porous hybrid inorganic/organic material, NaNi3(OH)(SIP)2 [SIP = 5-sulfoisophthalate][1], is shown to strongly bind molecular hydrogen at coordinatively unsaturated metal sites. A combination of H2 sorption isotherms, temperature programmed desorption, and inelastic neutron scattering spectroscopy show the existence of a considerable number of such strong binding sites in [1] along with other sites where hydrogen is more weakly physisorbed. The overall capacity for hydrogen of this material as well as the much stronger binding of hydrogen than in typical porous material represent an important step toward a possible utilization of porous media for hydrogen storage.
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Cited by
Kökçam-Demir, Ü., Goldman, A., Esrafili, L., Gharib, M., Morsali, A., Weingart, O., & Janiak, C. (2020) · Chemical Society Reviews · doi:10.1039/c9cs00609e · Cited by 895
Horike, S., Dincǎ, M., Tamaki, K., & Long, J. R. (2008) · Journal of the American Chemical Society · doi:10.1021/ja800669j · Cited by 834
Han, S. S., Mendoza-Cortés, J. L., & Goddard III, W. A. (2009) · Chemical Society Reviews · doi:10.1039/b802430h · Cited by 594
Systematic Functionalization of a Metal−Organic Framework via a Postsynthetic Modification Approach
Tanabe, K. K., Wang, Z., & Cohen, S. M. (2008) · Journal of the American Chemical Society · doi:10.1021/ja801848j · Cited by 386
Sumida, K., Horike, S., Kaye, S. S., Herm, Z. R., Queen, W. L., Brown, C. M., Grandjean, F., Long, G. J., Dailly, A., & Long, J. R. (2010) · Chemical Science · doi:10.1039/c0sc00179a · Cited by 347
Metadata
- Authors
- Forster, P. M., Eckert, J., Heiken, B. D., Parise, J. B., Yoon, J. W., Jhung, S. H., Chang, J.-S., & Cheetham, A. K.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2006-12-01
- Volume
- 128
- Issue
- 51
- Pages
- 16846-16850
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2078542319
- Cited by
- 198
- References
- 0
- FWCI
- 21.27
- Type
- journal article
- Language
- en
- Open access
- closed
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- Forster, P. M., Eckert, J., Heiken, B. D., Parise, J. B., Yoon, J. W., Jhung, S. H., Chang, J.-S., & Cheetham, A. K. (2006). Adsorption of Molecular Hydrogen on Coordinatively Unsaturated Ni(II) Sites in a Nanoporous Hybrid Material. Journal of the American Chemical Society. https://doi.org/10.1021/ja0649217
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