The DOI matches its Crossref record; 17 of the 17 references it cites were found in a registry or an index.
A General Synthetic Strategy for Oxide-Supported Metal Nanoparticle Catalysts
Abstract
Despite recent exciting progress in catalysis by supported gold nanoparticles, there remains the formidable challenge of preparing supported gold catalysts that collectively incorporate precise control over factors such as size and size-distribution of the gold nanoparticles, homogeneous dispersion of the particles on the support, and the ability to utilize a wide range of supports that profoundly affect catalytic performance. Here, we describe a synthetic methodology that achieves these goals. In this strategy, weak interface interactions evenly deposit presynthesized organic-capped metal nanoparticles on oxide supports. The homogeneous dispersion of nanoparticles on oxides is then locked in place, without aggregation, through careful calcination. The approach takes advantage of recent advances in the synthesis of metal and oxide nanomaterials and helps to bring together these two classes of materials for catalysis applications. An important feature is that the strategy allows metal nanoparticles to be well dispersed on a variety of oxides with few restrictions on their physical and chemical properties. Following this synthetic procedure, we have successfully developed efficient gold catalysts for green chemistry processes, such as the production of ethyl acetate from the selective oxidation of ethanol by oxygen at 100 degrees C.
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Cites
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Cited by
Correlating the Crystal Structure of A Thiol-Protected Au25 Cluster and Optical Properties
Zhu, M., Aikens, C. M., Hollander, F. J., Schatz, G. C., & Jin, R. (2008) · Journal of the American Chemical Society · doi:10.1021/ja801173r · Cited by 2,348
Nanoarchitectured Design of Porous Materials and Nanocomposites from Metal‐Organic Frameworks
Kaneti, Y. V., Tang, J., Salunkhe, R. R., Jiang, X., Yu, A., Wu, K. C. ‐., & Yamauchi, Y. (2017) · Advanced Materials · doi:10.1002/adma.201604898 · Cited by 888
Small particles, big impacts: A review of the diverse applications of nanofluids
Taylor, R., Coulombe, S., Otanicar, T., Phelan, P., Gunawan, A., Lv, W., Rosengarten, G., Prasher, R., & Tyagi, H. (2013) · Journal of Applied Physics · doi:10.1063/1.4754271 · Cited by 759
Selective oxidation using gold
Della Pina, C., Falletta, E., Prati, L., & Rossi, M. (2008) · Chemical Society Reviews · doi:10.1039/b707319b · Cited by 677
Tao, Y., Ju, E., Ren, J., & Qu, X. (2015) · Advanced Materials · doi:10.1002/adma.201405105 · Cited by 620
Metadata
- Authors
- Zheng, N., & Stucky, G. D.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2006-10-13
- Volume
- 128
- Issue
- 44
- Pages
- 14278-14280
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2163896356
- Cited by
- 502
- References
- 17
- FWCI
- 13.24
- Type
- journal article
- Language
- en
- Open access
- closed
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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