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Synthesis and Characterization of Ordered Intermetallic PtPb Nanorods
Abstract
We have demonstrated the synthesis of ordered intermetallic PtPb nanorods by simultaneously reducing platinum acetylacetonate and lead acetylacetonate with a tert -butylamine−borane complex in a mixture of diphenyl ether, adamantanecarboxylic acid, hexadecanethiol, and hexadecylamine. The formation of rodlike morphology is attributed to the preferable incorporation of Pt and Pb adatoms onto sites with high-coordination numbers of the growing low-index surfaces based on a Kossel crystal analysis. These PtPb nanorods can be deposited onto carbon black and show high-catalytic properties toward methanol oxidation. The current mass density of this PtPb/C catalyst is above 700 mA mg -1 Pt, which is significantly higher than that of a commercial PtRu/C catalyst.
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Cites
Electrocatalytic Activity of Ordered Intermetallic Phases for Fuel Cell Applications
Casado-Rivera, E., Volpe, D. J., Alden, L., Lind, C., Downie, C., Vázquez-Alvarez, T., Angelo, A. C. D., DiSalvo, F. J., & Abruña, H. D. (2004) · Journal of the American Chemical Society · doi:10.1021/ja038497a · Cited by 521
Cited by
Biaxially strained PtPb/Pt core/shell nanoplate boosts oxygen reduction catalysis
Bu, L., Zhang, N., Guo, S., Zhang, X., Li, J., Yao, J., Wu, T., Lu, G., Ma, J.-Y., Su, D., et al. (2016) · Science · doi:10.1126/science.aah6133 · Cited by 1,642
Wang, Y.-J., Zhao, N., Fang, B., Li, H., Bi, X. T., & Wang, H. (2015) · Chemical Reviews · doi:10.1021/cr500519c · Cited by 1,267
Ethylene glycol: properties, synthesis, and applications
Yue, H., Zhao, Y., Ma, X., & Gong, J. (2012) · Chemical Society Reviews · doi:10.1039/c2cs15359a · Cited by 1,180
Peng, Z., & Yang, H. (2009) · Nano Today · doi:10.1016/j.nantod.2008.10.010 · Cited by 1,085
Self-citationTruncated Octahedral Pt3Ni Oxygen Reduction Reaction Electrocatalysts
Wu, J., Zhang, J., Peng, Z., Yang, S., Wagner, F. T., & Yang, H. (2010) · Journal of the American Chemical Society · doi:10.1021/ja100571h · Cited by 520
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Metadata
- Authors
- Maksimuk, S., Yang, S., Peng, Z., & Yang, H.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2007-06-20
- Volume
- 129
- Issue
- 28
- Pages
- 8684-8685
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2092764862
- Cited by
- 167
- References
- 1
- FWCI
- 9.93
- Type
- journal article
- Language
- en
- Open access
- closed
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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