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Reticular Synthesis of Microporous and Mesoporous 2D Covalent Organic Frameworks
Abstract
Three new crystalline microporous and mesoporous 2D covalent organic frameworks termed COF-6, -8, and -10 from boronic acid building blocks and 2,3,6,7,10,11-hexahydroxytriphenylene have been synthesized and structurally characterized. These materials constructed of C 2 O 2 B rings form eclipsed layered structures with pore sizes ranging from 6.4 to 34.1 Å and are found to have high thermal stability, low density, and high porosity as indicated by the surface areas of 980, 1400, and 2080 m 2 g -1 for COF-6, -8, and -10, respectively. The control of pore size and structure demonstrates the effectiveness of reticular chemistry methods toward materials design.
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Citations
Cited by
Stable, crystalline, porous, covalent organic frameworks as a platform for chiral organocatalysts
Xu, H., Gao, J., & Jiang, D. (2015) · Nature Chemistry · doi:10.1038/nchem.2352 · Cited by 1,643
Covalent Organic Framework Photocatalysts: Structures and Applications
Wang, H., Wang, H., Wang, Z., Tang, L., Zeng, G., Xu, P., Chen, M., Xiong, T., Zhou, C., Li, X., et al. (2020) · Chemical Society Reviews · doi:10.1039/d0cs00278j · Cited by 1,301
Liu, R., Tan, K. T., Gong, Y., Chen, Y., Li, Z., Xie, S., He, T., Lu, Z., Yang, H., & Jiang, D. (2021) · Chemical Society Reviews · doi:10.1039/d0cs00620c · Cited by 1,083
Wang, H., Zeng, Z., Xu, P., Li, L., Zeng, G., Xiao, R., Tang, Z., Huang, D., Tang, L., Lai, C., et al. (2019) · Chemical Society Reviews · doi:10.1039/c8cs00376a · Cited by 804
Two‐Dimensional Polymers: Just a Dream of Synthetic Chemists?
Sakamoto, J., van Heijst, J., Lukin, O., & Schlüter, A. D. (2009) · Angewandte Chemie International Edition · doi:10.1002/anie.200801863 · Cited by 734
Metadata
- Authors
- Côté, A. P., El-Kaderi, H. M., Furukawa, H., Hunt, J. R., & Yaghi, O. M.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2007-10-01
- Volume
- 129
- Issue
- 43
- Pages
- 12914-12915
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2044944060
- Cited by
- 812
- References
- 0
- FWCI
- 20.48
- Type
- journal article
- Language
- en
- Open access
- closed
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- Côté, A. P., El-Kaderi, H. M., Furukawa, H., Hunt, J. R., & Yaghi, O. M. (2007). Reticular Synthesis of Microporous and Mesoporous 2D Covalent Organic Frameworks. Journal of the American Chemical Society. https://doi.org/10.1021/ja0751781
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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