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Metal−Organic Polyhedral Frameworks: High H2 Adsorption Capacities and Neutron Powder Diffraction Studies
Abstract
Neutron powder diffraction experiments on D(2)-loaded NOTT-112 reveal that the axial sites of exposed Cu(II) ions in the smallest cuboctahedral cages are the first, strongest binding sites for D(2) leading to an overall discrimination between the two types of exposed Cu(II) sites at the paddlewheel nodes. Thus, the Cu(II) centers within the cuboctahedral cage are the first sites of D(2) binding with a Cu-D(2) distance of 2.23(1) A.
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Metadata
- Authors
- Yan, Y., Telepeni, I., Yang, S., Lin, X., Kockelmann, W., Dailly, A., Blake, A. J., Lewis, W., Walker, G. S., Allan, D. R., Barnett, S. A., Champness, N. R., & Schröder, M.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2010-03-03
- Volume
- 132
- Issue
- 12
- Pages
- 4092-4094
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2072587093
- Cited by
- 291
- References
- 0
- FWCI
- 25.24
- Type
- journal article
- Language
- en
- Open access
- closed
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