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Atomic-Level Pd−Pt Alloying and Largely Enhanced Hydrogen-Storage Capacity in Bimetallic Nanoparticles Reconstructed from Core/Shell Structure by a Process of Hydrogen Absorption/Desorption
Abstract
We have achieved the creation of a solid-solution alloy where Pd and Pt are homogeneously mixed at the atomic level, by a process of hydrogen absorption/desorption as a trigger for core (Pd)/shell (Pt) nanoparticles. The structural change from core/shell to solid solution has been confirmed by in situ powder X-ray diffraction, energy dispersive spectra, solid-state (2)H NMR measurement, and hydrogen pressure-composition isotherms. The successfully obtained Pd-Pt solid-solution nanoparticles with a Pt content of 8-21 atom % had a higher hydrogen-storage capacity than Pd nanoparticles. Moreover, the hydrogen-storage capacity of Pd-Pt solid-solution nanoparticles can be tuned by changing the composition of Pd and Pt.
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Nanoalloys: From Theory to Applications of Alloy Clusters and Nanoparticles
Ferrando, R., Jellinek, J., & Johnston, R. L. (2008) · Chemical Reviews · doi:10.1021/cr040090g · Cited by 3,690
Cited by
Kusada, K., Kobayashi, H., Ikeda, R., Kubota, Y., Takata, M., Toh, S., Yamamoto, T., Matsumura, S., Sumi, N., Sato, K., et al. (2014) · Journal of the American Chemical Society · doi:10.1021/ja409464g · Cited by 275
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Metadata
- Authors
- Kobayashi, H., Yamauchi, M., Kitagawa, H., Kubota, Y., Kato, K., & Takata, M.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2010-04-02
- Volume
- 132
- Issue
- 16
- Pages
- 5576-5577
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W1999862699
- Cited by
- 159
- References
- 1
- FWCI
- 6.80
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: Atomic-Level Pd−Pt Alloying and Largely Enhanced Hydrogen-Storage Capacity in Bimetallic Nanoparticles Reconstructed from Core/Shell Structure by a Process of Hydrogen Absorption/Desorption. https://app.cochat.ai/papers/10.1021/ja1013163
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- Kobayashi, H., Yamauchi, M., Kitagawa, H., Kubota, Y., Kato, K., & Takata, M. (2010). Atomic-Level Pd−Pt Alloying and Largely Enhanced Hydrogen-Storage Capacity in Bimetallic Nanoparticles Reconstructed from Core/Shell Structure by a Process of Hydrogen Absorption/Desorption. Journal of the American Chemical Society. https://doi.org/10.1021/ja1013163
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
