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SnSe Nanocrystals: Synthesis, Structure, Optical Properties, and Surface Chemistry
Abstract
The colloidal synthesis of SnSe nanoparticles is accomplished through the injection of bis[bis(trimethylsilyl)amino]tin(II) into hot trioctylphosphine:selenium in the presence of oleylamine. Through the manipulation of reaction temperature particles are grown with the average diameter reliably tuned to 4-10 nm. Quantum confinement is examined by establishing a relationship between particle size and band gap while the in depth growth dynamics are illuminated through UV-vis-NIR spectroscopy. Surface chemistry effects are explored, including the demonstration of useful ligand exchanges and the development of routes toward anisotropic particle growth. Finally, transient current-voltage properties of SnSe nanocrystal films in the dark and light are examined.
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Cited by
Implicit solvation model for density-functional study of nanocrystal surfaces and reaction pathways
Mathew, K., Sundararaman, R., Letchworth-Weaver, K., Arias, T. A., & Hennig, R. G. (2014) · The Journal of Chemical Physics · doi:10.1063/1.4865107 · Cited by 3,196
Gao, M.-R., Xu, Y.-F., Jiang, J., & Yu, S.-H. (2013) · Chemical Society Reviews · doi:10.1039/c2cs35310e · Cited by 1,610
Guo, R., Wang, X., Kuang, Y., & Huang, B. (2015) · Physical Review B · doi:10.1103/physrevb.92.115202 · Cited by 527
Size/Shape-Controlled Synthesis of Colloidal CdSe Quantum Disks: Ligand and Temperature Effects
Li, Z., & Peng, X. (2011) · Journal of the American Chemical Society · doi:10.1021/ja108145c · Cited by 299
Metadata
- Authors
- Baumgardner, W. J., Choi, J. J., Lim, Y.-F., & Hanrath, T.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2010-06-28
- Volume
- 132
- Issue
- 28
- Pages
- 9519-9521
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2055483946
- Cited by
- 307
- References
- 0
- FWCI
- 9.88
- Type
- journal article
- Language
- en
- Open access
- closed
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- Baumgardner, W. J., Choi, J. J., Lim, Y.-F., & Hanrath, T. (2010). SnSe Nanocrystals: Synthesis, Structure, Optical Properties, and Surface Chemistry. Journal of the American Chemical Society. https://doi.org/10.1021/ja1013745
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