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Synthetic Control of Structural Order in N-Alkylthieno[3,4-c]pyrrole-4,6-dione-Based Polymers for Efficient Solar Cells
Abstract
The correlation between the nature of alkyl substituents on N-alkylthieno[3,4-c]pyrrole-4,6-dione (TPD)-based polymers and solar cell device performance has been investigated. After adjusting device parameters, these TPD-based polymers used with PC(61)BM provided photovoltaic responses ranging from 4.0% to 6.8%, depending on the size and shape of the alkyl solubilizing groups. Further, we have correlated the effect of the alkyl groups on the structural order and orientation of the polymer backbone using grazing incidence X-ray scattering analysis, and we have demonstrated how fine-tuning of these parameters can improve the power conversion efficiency.
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Cited by
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Guo, X., Zhou, N., Lou, S. J., Smith, J., Tice, D. B., Hennek, J. W., Ortiz, R. P., Navarrete, J. T. L., Li, S., Strzalka, J., et al. (2013) · Nature Photonics · doi:10.1038/nphoton.2013.207 · Cited by 938
Dang, M. T., Hirsch, L., Wantz, G., & Wuest, J. D. (2013) · Chemical Reviews · doi:10.1021/cr300005u · Cited by 587
Yiu, A. T., Beaujuge, P. M., Lee, O. P., Woo, C. H., Toney, M. F., & Fréchet, J. M. J. (2012) · Journal of the American Chemical Society · doi:10.1021/ja2089662 · Cited by 491
Self-citationSilver nanowire-polymer composite electrodes for efficient polymer solar cells
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Meager, I., Ashraf, R. S., Mollinger, S., Schroeder, B. C., Bronstein, H., Beatrup, D., Vezie, M. S., Kirchartz, T., Salleo, A., Nelson, J., et al. (2013) · Journal of the American Chemical Society · doi:10.1021/ja406934j · Cited by 274
Metadata
- Authors
- Piliego, C., Holcombe, T. W., Douglas, J. D., Woo, C. H., Beaujuge, P. M., & Fréchet, J. M. J.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2010-05-14
- Volume
- 132
- Issue
- 22
- Pages
- 7595-7597
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W1969325537
- Cited by
- 907
- References
- 0
- FWCI
- 116.37
- Type
- journal article
- Language
- en
- Open access
- closed
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- Piliego, C., Holcombe, T. W., Douglas, J. D., Woo, C. H., Beaujuge, P. M., & Fréchet, J. M. J. (2010). Synthetic Control of Structural Order in N-Alkylthieno[3,4-c]pyrrole-4,6-dione-Based Polymers for Efficient Solar Cells. Journal of the American Chemical Society. https://doi.org/10.1021/ja103275u
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