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Large-Area Graphene Single Crystals Grown by Low-Pressure Chemical Vapor Deposition of Methane on Copper
Abstract
Graphene single crystals with dimensions of up to 0.5 mm on a side were grown by low-pressure chemical vapor deposition in copper-foil enclosures using methane as a precursor. Low-energy electron microscopy analysis showed that the large graphene domains had a single crystallographic orientation, with an occasional domain having two orientations. Raman spectroscopy revealed the graphene single crystals to be uniform monolayers with a low D-band intensity. The electron mobility of graphene films extracted from field-effect transistor measurements was found to be higher than 4000 cm(2) V(-1) s(-1) at room temperature.
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Citations
Cited by
Progress, Challenges, and Opportunities in Two-Dimensional Materials Beyond Graphene
Butler, S. Z., Hollen, S. M., Cao, L., Cui, Y., Gupta, J. A., Gutiérrez, H. R., Heinz, T. F., Hong, S. S., Huang, J., Ismach, A. F., et al. (2013) · ACS Nano · doi:10.1021/nn400280c · Cited by 4,878
Self-citationElectrochemistry of Graphene and Related Materials
Ambrosi, A., Chua, C. K., Bonanni, A., & Pumera, M. (2014) · Chemical Reviews · doi:10.1021/cr500023c · Cited by 1,208
Graphene synthesis: relationship to applications
Edwards, R. S., & Coleman, K. S. (2013) · Nanoscale · doi:10.1039/c2nr32629a · Cited by 773
Zeng, M., Xiao, Y., Liu, J., Yang, K., & Fu, L. (2018) · Chemical Reviews · doi:10.1021/acs.chemrev.7b00633 · Cited by 574
Effects of Polycrystalline Cu Substrate on Graphene Growth by Chemical Vapor Deposition
Wood, J. D., Schmucker, S. W., Lyons, A. S., Pop, E., & Lyding, J. W. (2011) · Nano Letters · doi:10.1021/nl201566c · Cited by 470
Metadata
- Authors
- Li, X., Magnuson, C. W., Venugopal, A., Tromp, R. M., Hannon, J. B., Vogel, E. M., Colombo, L., & Ruoff, R. S.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2011-02-10
- Volume
- 133
- Issue
- 9
- Pages
- 2816-2819
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2064286028
- Cited by
- 1,274
- References
- 0
- FWCI
- 65.38
- Type
- journal article
- Language
- en
- Open access
- closed
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- Li, X., Magnuson, C. W., Venugopal, A., Tromp, R. M., Hannon, J. B., Vogel, E. M., Colombo, L., & Ruoff, R. S. (2011). Large-Area Graphene Single Crystals Grown by Low-Pressure Chemical Vapor Deposition of Methane on Copper. Journal of the American Chemical Society. https://doi.org/10.1021/ja109793s
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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