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Wide Control of Proton Conductivity in Porous Coordination Polymers
Abstract
The proton conductivities of the porous coordination polymers M(OH)(bdc-R) [H(2)bdc = 1,4-benzenedicarboxylic acid; M = Al, Fe; R = H, NH(2), OH, (COOH)(2)] were investigated under humid conditions. Good correlations among pK(a), proton conductivity, and activation energy were observed. Fe(OH)(bdc-(COOH)(2)), having carboxy group and the lowest pK(a), showed the highest proton conductivity and the lowest activation energy in this system. This is the first example in which proton conductivity has been widely controlled by substitution of ligand functional groups in an isostructural series.
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Cited by
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Furukawa, H., Cordova, K. E., O’Keeffe, M., & Yaghi, O. M. (2013) · Science · doi:10.1126/science.1230444 · Cited by 16,945
Water Stability and Adsorption in Metal–Organic Frameworks
Burtch, N. C., Jasuja, H., & Walton, K. S. (2014) · Chemical Reviews · doi:10.1021/cr5002589 · Cited by 2,730
Water adsorption in MOFs: fundamentals and applications
Canivet, J., Fateeva, A., Guo, Y., Coasne, B., & Farrusseng, D. (2014) · Chem. Soc. Rev. · doi:10.1039/c4cs00078a · Cited by 1,444
Metal–organic frameworks as platforms for clean energy
Li, S.-L., & Xu, Q. (2013) · Energy & Environmental Science · doi:10.1039/c3ee40507a · Cited by 970
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Morozan, A., & Jaouen, F. (2012) · Energy & Environmental Science · doi:10.1039/c2ee22989g · Cited by 870
Metadata
- Authors
- Shigematsu, A., Yamada, T., & Kitagawa, H.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2011-02-01
- Volume
- 133
- Issue
- 7
- Pages
- 2034-2036
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2316441214
- Cited by
- 661
- References
- 0
- FWCI
- 26.62
- Type
- journal article
- Language
- en
- Open access
- closed
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