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Electrochemical Unzipping of Multi-walled Carbon Nanotubes for Facile Synthesis of High-Quality Graphene Nanoribbons
Abstract
Here we report a remarkable transformation of carbon nanotubes (CNTs) to nanoribbons composed of a few layers of graphene by a two-step electrochemical approach. This consists of the oxidation of CNTs at controlled potential, followed by reduction to form graphene nanoribbons (GNRs) having smooth edges and fewer defects, as evidenced by multiple characterization techniques, including Raman spectroscopy, atomic force microscopy, and transmission electron microscopy. This type of "unzipping" of CNTs (single-walled, multi-walled) in the presence of an interfacial electric field provides unique advantages with respect to the orientation of CNTs, which might make possible the production of GNRs with controlled widths and fewer defects.
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Citations
Cites
Two-dimensional gas of massless Dirac fermions in graphene
Novoselov, K. S., Geim, A. K., Morozov, S. V., Jiang, D., Katsnelson, M. I., Grigorieva, I. V., Dubonos, S. V., & Firsov, A. A. (2005) · Nature · doi:10.1038/nature04233 · Cited by 21,611
Narrow graphene nanoribbons from carbon nanotubes
Jiao, L., Zhang, L., Wang, X., Diankov, G., & Dai, H. (2009) · Nature · doi:10.1038/nature07919 · Cited by 2,441
Cited by
Kumar, R., Sahoo, S., Joanni, E., Singh, R. K., Tan, W. K., Kar, K. K., & Matsuda, A. (2019) · Progress in Energy and Combustion Science · doi:10.1016/j.pecs.2019.100786 · Cited by 554
Recent developments in 2D layered inorganic nanomaterials for sensing
Kannan, P. K., Late, D. J., Morgan, H., & Rout, C. S. (2015) · Nanoscale · doi:10.1039/c5nr03633j · Cited by 454
Kumar, R., Singh, R. K., Singh, D. P., Joanni, E., Yadav, R. M., & Moshkalev, S. A. (2017) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2017.03.021 · Cited by 299
Metadata
- Authors
- Shinde, D. B., Debgupta, J., Kushwaha, A., Aslam, M., & Pillai, V. K.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2011-03-09
- Volume
- 133
- Issue
- 12
- Pages
- 4168-4171
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2091548978
- Cited by
- 225
- References
- 2
- FWCI
- 10.07
- Type
- journal article
- Language
- en
- Open access
- closed
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- Shinde, D. B., Debgupta, J., Kushwaha, A., Aslam, M., & Pillai, V. K. (2011). Electrochemical Unzipping of Multi-walled Carbon Nanotubes for Facile Synthesis of High-Quality Graphene Nanoribbons. Journal of the American Chemical Society. https://doi.org/10.1021/ja1101739
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
