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Metal-Free Activation of Dioxygen by Graphene/g-C3N4Nanocomposites: Functional Dyads for Selective Oxidation of Saturated Hydrocarbons
Abstract
Graphene sheet/polymeric carbon nitride nanocomposite (GSCN) functions as a metal-free catalyst to activate O(2) for the selective oxidation of secondary C-H bonds of cyclohexane. By fine-tuning the weight ratio of graphene and carbon nitride components, GSCN offers good conversion and high selectivity to corresponding ketones. Besides its high stability, this catalyst also exhibits high chemoselectivity for secondary C-H bonds of various saturated alkanes and, therefore, should be useful in overcoming challenges confronted by metal-mediated catalysis.
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Cites
Geim, A. K., & Novoselov, K. S. (2007) · Nature Materials · doi:10.1038/nmat1849 · Cited by 39,979
Cited by
Ong, W.-J., Tan, L.-L., Ng, Y. H., Yong, S.-T., & Chai, S.-P. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00075 · Cited by 7,147
Progress, challenge and perspective of heterogeneous photocatalysts
Qu, Y., & Duan, X. (2013) · Chem. Soc. Rev. · doi:10.1039/c2cs35355e · Cited by 1,466
Dong, G., Zhang, Y., Pan, Q., & Qiu, J. (2014) · Journal of Photochemistry and Photobiology C: Photochemistry Reviews · doi:10.1016/j.jphotochemrev.2014.04.002 · Cited by 1,085
Zeng, M., Xiao, Y., Liu, J., Yang, K., & Fu, L. (2018) · Chemical Reviews · doi:10.1021/acs.chemrev.7b00633 · Cited by 574
Xiao, X., Gao, Y., Zhang, L., Zhang, J., Zhang, Q., Li, Q., Bao, H., Zhou, J., Miao, S., Chen, N., et al. (2020) · Advanced Materials · doi:10.1002/adma.202003082 · Cited by 528
Yang, M.-Q., Zhang, N., & Xu, Y.-J. (2013) · ACS Applied Materials & Interfaces · doi:10.1021/am3029798 · Cited by 365
Patel, M. A., Luo, F., Khoshi, M. R., Rabie, E., Zhang, Q., Flach, C. R., Mendelsohn, R., Garfunkel, E., Szostak, M., & He, H. (2016) · ACS Nano · doi:10.1021/acsnano.5b07054 · Cited by 359
Recent progress on graphene-based hybrid electrocatalysts
Xia, B., Yan, Y., Wang, X., & Lou, X. W. (. (2014) · Mater. Horiz. · doi:10.1039/c4mh00040d · Cited by 331
Self-citationCheng, F., Wang, H., & Dong, X. (2015) · Chemical Communications · doi:10.1039/c5cc01035g · Cited by 255
Ge, J.-M., Zhang, B., Lv, L.-B., Wang, H.-H., Ye, T.-N., Wei, X., Su, J., Wang, K.-X., Li, X.-H., & Chen, J.-S. (2015) · Nano Energy · doi:10.1016/j.nanoen.2015.05.017 · Cited by 60
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Metadata
- Authors
- Li, X.-H., Chen, J.-S., Wang, X., Sun, J., & Antonietti, M.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2011-05-11
- Volume
- 133
- Issue
- 21
- Pages
- 8074-8077
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W1995554639
- Cited by
- 524
- References
- 1
- FWCI
- 15.41
- Type
- journal article
- Language
- en
- Open access
- closed
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