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One-Pot Catalytic Conversion of Cellulose and of Woody Biomass Solids to Liquid Fuels
Open accessAbstract
Efficient methodologies for converting biomass solids to liquid fuels have the potential to reduce dependence on imported petroleum while easing the atmospheric carbon dioxide burden. Here, we report quantitative catalytic conversions of wood and cellulosic solids to liquid and gaseous products in a single stage reactor operating at 300-320 °C and 160-220 bar. Little or no char is formed during this process. The reaction medium is supercritical methanol (sc-MeOH) and the catalyst, a copper-doped porous metal oxide, is composed of earth-abundant materials. The major liquid product is a mixture of C(2)-C(6) aliphatic alcohols and methylated derivatives thereof that are, in principle, suitable for applications as liquid fuels.
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Cites
The Catalytic Valorization of Lignin for the Production of Renewable Chemicals
Zakzeski, J., Bruijnincx, P. C. A., Jongerius, A. L., & Weckhuysen, B. M. (2010) · Chemical Reviews · doi:10.1021/cr900354u · Cited by 4,468
Cited by
Wu, X., Fan, X., Xie, S., Lin, J., Cheng, J., Zhang, Q., Chen, L., & Wang, Y. (2018) · Nature Catalysis · doi:10.1038/s41929-018-0148-8 · Cited by 649
Current challenges in commercially producing biofuels from lignocellulosic biomass
Balan, V. (2014) · ISRN Biotechnology · doi:10.1155/2014/463074 · Cited by 551
Lignin depolymerization into aromatic monomers over solid acid catalysts
Deepa, A. K., & Dhepe, P. L. (2015) · ACS Catalysis · doi:10.1021/cs501371q · Cited by 346
Depolymerization of lignin via a non-precious Ni–Fe alloy catalyst supported on activated carbon
Zhai, Y., Li, C., Xu, G., Ma, Y., Liu, X., & Zhang, Y. (2017) · Green Chemistry · doi:10.1039/c7gc00149e · Cited by 249
Wang, C., Zhang, X., Liu, Q., Zhang, Q., Chen, L., & Ma, L. (2020) · Fuel Processing Technology · doi:10.1016/j.fuproc.2020.106485 · Cited by 157
Metadata
- Authors
- Matson, T. D., Barta, K., Iretskii, A. V., & Ford, P. C.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2011-08-17
- Volume
- 133
- Issue
- 35
- Pages
- 14090-14097
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W1982599553
- Cited by
- 345
- References
- 1
- FWCI
- 10.03
- Type
- journal article
- Language
- en
- Open access
- green
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- Matson, T. D., Barta, K., Iretskii, A. V., & Ford, P. C. (2011). One-Pot Catalytic Conversion of Cellulose and of Woody Biomass Solids to Liquid Fuels. Journal of the American Chemical Society. https://doi.org/10.1021/ja205436c
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
