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Efficient Synthesis of Single Gold Nanoparticle Hybrid Amphiphilic Triblock Copolymers and Their Controlled Self-Assembly
Abstract
We report on a robust approach to the size-selective and template-free synthesis of asymmetrically functionalized ultrasmall (<4 nm) gold nanoparticles (AuNPs) stably anchored with a single amphiphilic triblock copolymer chain per NP. Directed NP self-assembly in aqueous solution can be facilely accomplished to afford organic/inorganic hybrid micelles, vesicles, rods, and large compound micelles by taking advantage of the rich microphase separation behavior of the as-synthesized AuNP hybrid amphiphilic triblock copolymers, PEO-AuNP-PS, which act as the polymer-metal-polymer analogue of conventional amphiphilic triblock copolymers. Factors affecting the size-selective fabrication and self-assembly characteristics and the time-dependent morphological evolution of NP assemblies were thoroughly explored.
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Blanazs, A., Armes, S. P., & Ryan, A. J. (2009) · Macromolecular Rapid Communications · doi:10.1002/marc.200800713 · Cited by 1,500
Origins of complex self-assembly in block copolymers
Matsen, M. W., & Bates, F. S. (1996) · Macromolecules · doi:10.1021/ma960744q · Cited by 578
Cited by
Song, J., Zhou, J., & Duan, H. (2012) · Journal of the American Chemical Society · doi:10.1021/ja305154a · Cited by 438
Amphiphile nanoarchitectonics: from basic physical chemistry to advanced applications
Ramanathan, M., Shrestha, L. K., Mori, T., Ji, Q., Hill, J. P., & Ariga, K. (2013) · Physical Chemistry Chemical Physics · doi:10.1039/c3cp50620g · Cited by 353
Metadata
- Authors
- Hu, J., Wu, T., Zhang, G., & Liu, S.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2012-04-30
- Volume
- 134
- Issue
- 18
- Pages
- 7624-7627
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2316494100
- Cited by
- 165
- References
- 2
- FWCI
- 10.94
- Type
- journal article
- Language
- en
- Open access
- closed
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- Hu, J., Wu, T., Zhang, G., & Liu, S. (2012). Efficient Synthesis of Single Gold Nanoparticle Hybrid Amphiphilic Triblock Copolymers and Their Controlled Self-Assembly. Journal of the American Chemical Society. https://doi.org/10.1021/ja302019q
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