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Highly Stable Water Splitting on Oxynitride TaON Photoanode System under Visible Light Irradiation
Abstract
Highly stable photoelectrochemical water splitting is demonstrated for the first time on a tantalum oxynitride (TaON) photoanode under visible light irradiation. Highly dispersed CoO(x) nanoparticles on the TaON photoanode efficiently scavenge photogenerated holes and effectively suppress self-oxidative deactivation of the TaON surface, resulting in a stable photocurrent. The use of highly dispersed CoO(x) cocatalyst on TaON together with phosphate solutions significantly increased the photocurrent due to the formation of a cobalt/phosphate phase. This enabled us to stably split water into H(2) and O(2) under visible light irradiation at a relatively low applied bias (0.6 V vs Pt counter electrode).
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Abe, R. (2010) · Journal of Photochemistry and Photobiology C: Photochemistry Reviews · doi:10.1016/j.jphotochemrev.2011.02.003 · Cited by 1,223
Self-citation
Cited by
Roles of Cocatalysts in Photocatalysis and Photoelectrocatalysis
Yang, J., Wang, D., Han, H., & Li, C. (2013) · Accounts of Chemical Research · doi:10.1021/ar300227e · Cited by 2,848
Visible-light driven heterojunction photocatalysts for water splitting – a critical review
Moniz, S. J. A., Shevlin, S. A., Martin, D. J., Guo, Z.-X., & Tang, J. (2015) · Energy & Environmental Science · doi:10.1039/c4ee03271c · Cited by 2,363
Semiconducting materials for photoelectrochemical energy conversion
Sivula, K., & van de Krol, R. (2016) · Nature Reviews Materials · doi:10.1038/natrevmats.2015.10 · Cited by 1,645
Wang, Y., Suzuki, H., Xie, J., Tomita, O., Martin, D. J., Higashi, M., Kong, D., Abe, R., & Tang, J. (2018) · Chemical Reviews · doi:10.1021/acs.chemrev.7b00286 · Cited by 1,043
Self-citationPhotocurrent of BiVO4 is limited by surface recombination, not surface catalysis
Zachäus, C., Abdi, F. F., Peter, L. M., & van de Krol, R. (2017) · Chemical Science · doi:10.1039/c7sc00363c · Cited by 549
Metadata
- Authors
- Higashi, M., Domen, K., & Abe, R.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2012-04-12
- Volume
- 134
- Issue
- 16
- Pages
- 6968-6971
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2012177248
- Cited by
- 418
- References
- 1
- FWCI
- 15.43
- Type
- journal article
- Language
- en
- Open access
- closed
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