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Pore Surface Engineering with Controlled Loadings of Functional Groups via Click Chemistry in Highly Stable Metal–Organic Frameworks
Abstract
Reactions of ZrCl(4) and single or mixed linear dicarboxylic acids bearing methyl or azide groups lead to highly stable isoreticular metal-organic frameworks (MOFs) with content-tunable, accessible, reactive azide groups inside the large pores. These Zr-based MOFs offer an ideal platform for pore surface engineering by anchoring various functional groups with controlled loadings onto the pore walls via the click reaction, endowing the MOFs with tailor-made interfaces. Significantly, the framework and crystallinity of the functionalized MOFs are well-retained, and the engineered pore surfaces have been demonstrated to be readily accessible, thus providing more opportunities for powerful and broad applications of MOFs.
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Horike, S., Shimomura, S., & Kitagawa, S. (2009) · Nature Chemistry · doi:10.1038/nchem.444 · Cited by 2,486
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Burtch, N. C., Jasuja, H., & Walton, K. S. (2014) · Chemical Reviews · doi:10.1021/cr5002589 · Cited by 2,730
Wu, H., Chua, Y. S., Krungleviciute, V., Tyagi, M., Chen, P., Yildirim, T., & Zhou, W. (2013) · Journal of the American Chemical Society · doi:10.1021/ja404514r · Cited by 1,457
From fundamentals to applications: a toolbox for robust and multifunctional MOF materials
Kirchon, A., Feng, L., Drake, H. F., Joseph, E. A., & Zhou, H.-C. (2018) · Chemical Society Reviews · doi:10.1039/c8cs00688a · Cited by 1,448
Self-citationWei, Z., Gu, Z.-Y., Arvapally, R. K., Chen, Y.-P., McDougald, R. N., Ivy, J. F., Yakovenko, A. A., Feng, D., Omary, M. A., & Zhou, H.-C. (2014) · Journal of the American Chemical Society · doi:10.1021/ja5006866 · Cited by 657
Self-citationMetal-organic frameworks as novel matrices for efficient enzyme immobilization: An update review
Liang, S., Wu, X.-L., Xiong, J., Zong, M.-H., & Lou, W.-Y. (2020) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2019.213149 · Cited by 441
Metadata
- Authors
- Jiang, H.-L., Feng, D., Liu, T.-F., Li, J.-R., & Zhou, H.-C.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2012-08-27
- Volume
- 134
- Issue
- 36
- Pages
- 14690-14693
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2030971320
- Cited by
- 379
- References
- 1
- FWCI
- 20.80
- Type
- journal article
- Language
- en
- Open access
- closed
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