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Energy Transfer from Quantum Dots to Metal–Organic Frameworks for Enhanced Light Harvesting
Abstract
Because of their efficient energy-transport properties, porphyrin-based metal-organic frameworks (MOFs) are attractive compounds for solar photochemistry applications. However, their absorption bands provide limited coverage in the visible spectral range for light-harvesting applications. We report here the functionalization of porphyrin-based MOFs with CdSe/ZnS core/shell quantum dots (QDs) for the enhancement of light harvesting via energy transfer from the QDs to the MOFs. The broad absorption band of the QDs in the visible region offers greater coverage of the solar spectrum by QD-MOF hybrid structures. We show through time-resolved emission studies that photoexcitation of the QDs is followed by energy transfer to the MOFs with efficiencies of more than 80%. This sensitization approach can result in a >50% increase in the number of photons harvested by a single monolayer MOF structure with a monolayer of QDs on the surface of the MOF.
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Cites
Metal-organic framework materials as catalysts
Lee, J., Farha, O. K., Roberts, J., Scheidt, K. A., Nguyen, S. T., & Hupp, J. T. (2009) · Chemical Society Reviews · doi:10.1039/b807080f · Cited by 7,969
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Cited by
Metal–organic frameworks as platforms for clean energy
Li, S.-L., & Xu, Q. (2013) · Energy & Environmental Science · doi:10.1039/c3ee40507a · Cited by 970
Porous Metal–Organic Frameworks for Heterogeneous Biomimetic Catalysis
Zhao, M., Ou, S., & Wu, C.-D. (2014) · Accounts of Chemical Research · doi:10.1021/ar400265x · Cited by 722
MOF positioning technology and device fabrication
Falcaro, P., Ricco, R., Doherty, C. M., Liang, K., Hill, A. J., & Styles, M. J. (2014) · Chem. Soc. Rev. · doi:10.1039/c4cs00089g · Cited by 710
Photocatalytic Metal–Organic Framework from CdS Quantum Dot Incubated Luminescent Metallohydrogel
Saha, S., Das, G., Thote, J., & Banerjee, R. (2014) · Journal of the American Chemical Society · doi:10.1021/ja509019k · Cited by 365
Luminescent Metal–Organic Framework Films As Highly Sensitive and Fast-Response Oxygen Sensors
Dou, Z., Yu, J., Cui, Y., Yang, Y., Wang, Z., Yang, D., & Qian, G. (2014) · Journal of the American Chemical Society · doi:10.1021/ja411224j · Cited by 361
Metadata
- Authors
- Jin, S., Son, H.-J., Farha, O. K., Wiederrecht, G. P., & Hupp, J. T.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2013-01-14
- Volume
- 135
- Issue
- 3
- Pages
- 955-958
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2002926287
- Cited by
- 358
- References
- 1
- FWCI
- 23.57
- Type
- journal article
- Language
- en
- Open access
- closed
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- Jin, S., Son, H.-J., Farha, O. K., Wiederrecht, G. P., & Hupp, J. T. (2013). Energy Transfer from Quantum Dots to Metal–Organic Frameworks for Enhanced Light Harvesting. Journal of the American Chemical Society. https://doi.org/10.1021/ja3097114
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