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Efficient Inorganic–Organic Hybrid Perovskite Solar Cells Based on Pyrene Arylamine Derivatives as Hole-Transporting Materials
Open accessAbstract
A set of three N,N-di-p-methoxyphenylamine-substituted pyrene derivatives have successfully been synthesized and characterized by (1)H/(13)C NMR spectroscopy, mass spectrometry, and elemental analysis. The optical and electronic structures of the pyrene derivatives were adjusted by controlling the ratio of N,N-di-p-methoxyphenylamine to pyrene, and investigated by UV/vis spectroscopy and cyclic voltammetry. The pyrene derivatives were employed as hole-transporting materials (HTMs) in fabricating mesoporous TiO2/CH3NH3PbI3/HTMs/Au solar cells. The pyrene-based derivative Py-C exhibited a short-circuit current density of 20.2 mA/cm(2), an open-circuit voltage (Voc) of 0.886 V, and a fill factor of 69.4% under an illumination of 1 sun (100 mW/cm(2)), resulting in an overall power conversion efficiency of 12.4%. The performance is comparable to that of the well-studied spiro-OMeTAD, even though the Voc is slightly lower. Thus, this newly synthesized pyrene derivative holds promise as a HTM for highly efficient perovskite-based solar cells.
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Cited by
Inorganic hole conductor-based lead halide perovskite solar cells with 12.4% conversion efficiency
Qin, P., Tanaka, S., Ito, S., Tetreault, N., Manabe, K., Nishino, H., Nazeeruddin, M. K., & Grätzel, M. (2014) · Nature Communications · doi:10.1038/ncomms4834 · Cited by 894
Self-citationo-Methoxy Substituents in Spiro-OMeTAD for Efficient Inorganic–Organic Hybrid Perovskite Solar Cells
Jeon, N. J., Lee, H. G., Kim, Y. C., Seo, J., Noh, J. H., Lee, J., & Seok, S. I. (2014) · Journal of the American Chemical Society · doi:10.1021/ja502824c · Cited by 787
Self-citationZhao, Y., & Zhu, K. (2014) · The Journal of Physical Chemistry C · doi:10.1021/jp502696w · Cited by 555
Yu, Z., & Sun, L. (2015) · Advanced Energy Materials · doi:10.1002/aenm.201500213 · Cited by 462
Advances in hole transport materials engineering for stable and efficient perovskite solar cells
Bakr, Z. H., Wali, Q., Fakharuddin, A., Schmidt-Mende, L., Brown, T. M., & Jose, R. (2017) · Nano Energy · doi:10.1016/j.nanoen.2017.02.025 · Cited by 455
Metadata
- Authors
- Jeon, N. J., Lee, J., Noh, J. H., Nazeeruddin, M. K., Grätzel, M., & Seok, S. I.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2013-12-12
- Volume
- 135
- Issue
- 51
- Pages
- 19087-19090
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2059675228
- Cited by
- 551
- References
- 0
- FWCI
- 46.33
- Type
- journal article
- Language
- en
- Open access
- green
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- Jeon, N. J., Lee, J., Noh, J. H., Nazeeruddin, M. K., Grätzel, M., & Seok, S. I. (2013). Efficient Inorganic–Organic Hybrid Perovskite Solar Cells Based on Pyrene Arylamine Derivatives as Hole-Transporting Materials. Journal of the American Chemical Society. https://doi.org/10.1021/ja410659k
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