The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Self-Supported PdxBi Catalysts for the Electrooxidation of Glycerol in Alkaline Media
Abstract
Highly active self-supported PdxBi catalysts are synthesized by the sacrificial support method. Self-supported PdxBi catalysts have a porous nanostructured morphology with high surface areas (in the range from 75 to 100 m(2) g(-1)), making PdxBi a state-of-the-art catalyst. Pd4Bi displays the highest activity toward glycerol oxidation. In situ Fourier transform infrared spectroscopy highlights the unique catalytic behavior of self-supported PdxBi materials due to their particular structure and morphology. The confinement of reactants and intermediates in pores acting as nanoreactors is responsible for the high selectivity as a function of the electrode potential: aldehyde and ketone at low potentials, hydroxypyruvate at moderate potentials, and CO2 at high potentials. Moreover, the selectivity depends on the electrode history: it is different for the positive potential scan direction than for the reverse direction, where the catalyst becomes selective toward the production of carboxylates.
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Cites
Platinum-Based Nanostructured Materials: Synthesis, Properties, and Applications
Chen, A., & Holt-Hindle, P. (2010) · Chemical Reviews · doi:10.1021/cr9003902 · Cited by 1,390
Electrocatalytic Activity of Ordered Intermetallic Phases for Fuel Cell Applications
Casado-Rivera, E., Volpe, D. J., Alden, L., Lind, C., Downie, C., Vázquez-Alvarez, T., Angelo, A. C. D., DiSalvo, F. J., & Abruña, H. D. (2004) · Journal of the American Chemical Society · doi:10.1021/ja038497a · Cited by 521
Shukla, A. K., Neergat, M., Bera, P., Jayaram, V, & Hegde, M. S. (2001) · Journal of Electroanalytical Chemistry · doi:10.1016/s0022-0728(01)00421-1 · Cited by 258
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Metadata
- Authors
- Zalineeva, A., Serov, A., Padilla, M., Martinez, U., Artyushkova, K., Baranton, S., Coutanceau, C., & Atanassov, P. B.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2014-02-27
- Volume
- 136
- Issue
- 10
- Pages
- 3937-3945
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2328839106
- Cited by
- 291
- References
- 3
- FWCI
- 10.04
- Type
- journal article
- Language
- en
- Open access
- closed
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