The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
Atomic Mechanism of Dynamic Electrochemical Lithiation Processes of MoS2 Nanosheets
Abstract
Layered molybdenum disulfide (MoS2) has been studied for decades for its diversity of structure and properties, where the structural dynamic evolution during lithium intercalation is an important but still indistinct, controversial topic. Here the electrochemical dynamic process of MoS2 nanosheets upon lithium intercalation has been systematically investigated by in situ high-resolution transmission electron microscopy. The results indicate that the lithiated MoS2 undergoes a trigonal prismatic (2H)-octahedral (1T) phase transition with a lithium ion occupying the interlayer S-S tetrahedron site in the 1T-LiMoS2. A pseudoperiodic structural modulation composed of polytype superlattices is also revealed as a consequence of the electron-lattice interaction. Furthermore, the shear mechanism of the 2H-1T phase transition has been confirmed by probing the dynamic phase boundary movement. The in situ real-time characterization at atomic scale provides a great leap forward in the fundamental understanding of the lithium ion storage mechanism in MoS2, which should be also of help for other transition metal dichalcogenides.
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Cites
Electronics and optoelectronics of two-dimensional transition metal dichalcogenides
Wang, Q. H., Kalantar-Zadeh, K., Kis, A., Coleman, J. N., & Strano, M. S. (2012) · Nature Nanotechnology · doi:10.1038/nnano.2012.193 · Cited by 16,374
The chemistry of two-dimensional layered transition metal dichalcogenide nanosheets
Chhowalla, M., Shin, H. S., Eda, G., Li, L.-J., Loh, K. P., & Zhang, H. (2013) · Nature Chemistry · doi:10.1038/nchem.1589 · Cited by 10,034
Cited by
Mahler, B., Hoepfner, V., Liao, K., & Ozin, G. A. (2014) · Journal of the American Chemical Society · doi:10.1021/ja506261t · Cited by 837
Zeng, M., Xiao, Y., Liu, J., Yang, K., & Fu, L. (2018) · Chemical Reviews · doi:10.1021/acs.chemrev.7b00633 · Cited by 574
Du, X., Huang, J., Zhang, J., Yan, Y., Wu, C., Hu, Y., Yan, C., Lei, T., Chen, W., Fan, C., et al. (2019) · Angewandte Chemie International Edition · doi:10.1002/anie.201810104 · Cited by 521
Schmidt, H., Giustiniano, F., & Eda, G. (2015) · Chemical Society Reviews · doi:10.1039/c5cs00275c · Cited by 466
Protein Induces Layer-by-Layer Exfoliation of Transition Metal Dichalcogenides
Guan, G., Zhang, S., Liu, S., Cai, Y., Low, M., Teng, C. P., Phang, I. Y., Cheng, Y., Duei, K. L., Srinivasan, B. M., et al. (2015) · Journal of the American Chemical Society · doi:10.1021/jacs.5b02780 · Cited by 426
Metadata
- Authors
- Wang, L., Xu, Z., Wang, W., & Bai, X.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2014-04-22
- Volume
- 136
- Issue
- 18
- Pages
- 6693-6697
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2103077907
- Cited by
- 526
- References
- 2
- FWCI
- 26.00
- Type
- journal article
- Language
- en
- Open access
- closed
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