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A Facile and General Coating Approach to Moisture/Water-Resistant Metal–Organic Frameworks with Intact Porosity
Abstract
The moisture sensitivity of many metal-organic frameworks (MOFs) poses a critical issue for their large-scale real application. One of the most effective methods to solve this problem is to convert the surface of MOFs from hydrophilic to hydrophobic. Herein, we develop a general strategy to modify hydrophobic polydimethysiloxane (PDMS) on the surface of MOF materials to significantly enhance their moisture or water resistance by a facile vapor deposition technique. MOF-5, HKUST-1, and ZnBT as representative vulnerable MOFs were successfully coated by PDMS, and these coated samples well inherited their original crystalline nature and pore characteristics. Strikingly, the surface areas of these MOFs were nearly 100% retained upon PDMS-coating. Such a coating process might render MOFs applicable in the presence of water or humidity in extended fields such as gas sorption and catalysis.
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Cites
Metal-organic framework materials as catalysts
Lee, J., Farha, O. K., Roberts, J., Scheidt, K. A., Nguyen, S. T., & Hupp, J. T. (2009) · Chemical Society Reviews · doi:10.1039/b807080f · Cited by 7,969
Cited by
Recent progress in metal-organic frameworks-based hydrogels and aerogels and their applications
Wang, L., Xu, H., Gao, J., Yao, J., & Zhang, Q. (2019) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2019.213016 · Cited by 594
Metal–Organic-Framework-Based Materials for Antimicrobial Applications
Li, R., Chen, T., & Pan, X. (2021) · ACS Nano · doi:10.1021/acsnano.0c09617 · Cited by 555
Understanding the Effect of Water on CO2 Adsorption
Kolle, J. M., Fayaz, M., & Sayari, A. (2021) · Chemical Reviews · doi:10.1021/acs.chemrev.0c00762 · Cited by 523
Al-Janabi, N., Hill, P., Torrente-Murciano, L., Garforth, A., Gorgojo, P., Siperstein, F., & Fan, X. (2015) · Chemical Engineering Journal · doi:10.1016/j.cej.2015.07.020 · Cited by 386
Metadata
- Authors
- Zhang, W., Hu, Y., Ge, J., Jiang, H.-L., & Yu, S.-H.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2014-11-24
- Volume
- 136
- Issue
- 49
- Pages
- 16978-16981
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W1968005961
- Cited by
- 588
- References
- 1
- FWCI
- 13.83
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhang, W., Hu, Y., Ge, J., Jiang, H.-L., & Yu, S.-H. (2014). A Facile and General Coating Approach to Moisture/Water-Resistant Metal–Organic Frameworks with Intact Porosity. Journal of the American Chemical Society. https://doi.org/10.1021/ja509960n
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
