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Rhombohedral Prussian White as Cathode for Rechargeable Sodium-Ion Batteries
Abstract
A novel air-stable sodium iron hexacyanoferrate (R-Na1.92Fe[Fe(CN)6]) with rhombohedral structure is demonstrated to be a scalable, low-cost cathode material for sodium-ion batteries exhibiting high capacity, long cycle life, and good rate capability. The cycling mechanism of the iron redox is clarified and understood through synchrotron-based soft X-ray absorption spectroscopy, which also reveals the correlation between the physical properties and the cell performance of this novel material. More importantly, successful preparation of a dehydrated iron hexacyanoferrate with high sodium-ion concentration enables the fabrication of a discharged sodium-ion battery with a non-sodium metal anode, and the manufacturing feasibility of low cost sodium-ion batteries with existing lithium-ion battery infrastructures has been tested.
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Citations
Cited by
Prussian Blue Analogs for Rechargeable Batteries
Wang, B., Han, Y., Wang, X., Bahlawane, N., Pan, H., Yan, M., & Jiang, Y. (2018) · iScience · doi:10.1016/j.isci.2018.04.008 · Cited by 499
Zuo, W., Luo, M., Liu, X., Wu, J., Liu, H., Li, J., Winter, M., Fu, R., Yang, W., & Yang, Y. (2020) · Energy & Environmental Science · doi:10.1039/d0ee01694b · Cited by 429
Self-citationA 30‐year overview of sodium‐ion batteries
Gao, Y., Zhang, H., Peng, J., Li, L., Xiao, Y., Li, L., Liu, Y., Qiao, Y., & Chou, S. (2024) · Carbon Energy · doi:10.1002/cey2.464 · Cited by 348
Chen, M., Liu, Q., Wang, S., Wang, E., Guo, X., & Chou, S. (2019) · Advanced Energy Materials · doi:10.1002/aenm.201803609 · Cited by 341
Wang, T., Su, D., Shanmukaraj, D., Rojo, T., Armand, M., & Wang, G. (2018) · Electrochemical Energy Reviews · doi:10.1007/s41918-018-0009-9 · Cited by 328
Metadata
- Authors
- Wang, L., Song, J., Qiao, R., Wray, L. A., Hossain, M. A., Chuang, Y.-D., Yang, W., Lu, Y., Evans, D., Lee, J.-J., Vail, S., Zhao, X., Nishijima, M., Kakimoto, S., & Goodenough, J. B.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-02-10
- Volume
- 137
- Issue
- 7
- Pages
- 2548-2554
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W1999429618
- Cited by
- 771
- References
- 0
- FWCI
- 29.67
- Type
- journal article
- Language
- en
- Open access
- closed
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- Wang, L., Song, J., Qiao, R., Wray, L. A., Hossain, M. A., Chuang, Y.-D., Yang, W., Lu, Y., Evans, D., Lee, J.-J., Vail, S., Zhao, X., Nishijima, M., Kakimoto, S., & Goodenough, J. B. (2015). Rhombohedral Prussian White as Cathode for Rechargeable Sodium-Ion Batteries. Journal of the American Chemical Society. https://doi.org/10.1021/ja510347s
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