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Photoelectrochemical Oxidation of Water Using BaTaO2N Photoanodes Prepared by Particle Transfer Method
Abstract
A photoanode of particulate BaTaO2N fabricated by the particle transfer method and modified with a Co cocatalyst generated a photocurrent of 4.2 mA cm(-2) at 1.2 V(RHE) in the photoelectrochemical water oxidation reaction under simulated sunlight (AM1.5G). The half-cell solar-to-hydrogen conversion efficiency (HC-STH) of the photoanode reached 0.7% at 1.0 V(RHE), which was an order of magnitude higher than the previously reported photoanode made from the same material. The faradaic efficiency for oxygen evolution from water was virtually 100% during the reaction for 6 h, attesting to the robustness of the oxynitride.
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Cites
Photocatalytic Water Splitting: Recent Progress and Future Challenges
Maeda, K., & Domen, K. (2010) · The Journal of Physical Chemistry Letters · doi:10.1021/jz1007966 · Cited by 2,739
Self-citationAbe, R. (2010) · Journal of Photochemistry and Photobiology C: Photochemistry Reviews · doi:10.1016/j.jphotochemrev.2011.02.003 · Cited by 1,223
Cited by
Semiconducting materials for photoelectrochemical energy conversion
Sivula, K., & van de Krol, R. (2016) · Nature Reviews Materials · doi:10.1038/natrevmats.2015.10 · Cited by 1,645
Metadata
- Authors
- Ueda, K., Minegishi, T., Clune, J., Nakabayashi, M., Hisatomi, T., Nishiyama, H., Katayama, M., Shibata, N., Kubota, J., Yamada, T., & Domen, K.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-02-06
- Volume
- 137
- Issue
- 6
- Pages
- 2227-2230
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2030779326
- Cited by
- 184
- References
- 2
- FWCI
- 7.92
- Type
- journal article
- Language
- en
- Open access
- closed
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- Ueda, K., Minegishi, T., Clune, J., Nakabayashi, M., Hisatomi, T., Nishiyama, H., Katayama, M., Shibata, N., Kubota, J., Yamada, T., & Domen, K. (2015). Photoelectrochemical Oxidation of Water Using BaTaO2N Photoanodes Prepared by Particle Transfer Method. Journal of the American Chemical Society. https://doi.org/10.1021/ja5131879
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