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Mechanistic Study of Photomediated Triangular Silver Nanoprism Growth
Open accessAbstract
This article presents a mechanistic study of the photomediated growth of silver nanoprisms. The data show that the photochemical process is driven by silver redox cycles involving reduction of silver cations by citrate on the silver particle surface and oxidative dissolution of small silver particles by O2. Bis(p-sulfonatophenyl)phenylphosphine increases the solubility of the Ag(+) by complexing it and acts as a buffer to keep the concentration of Ag(+) at 20 microM. The silver particles serve as photocatalysts and, under plasmon excitation, facilitate Ag(+) reduction by citrate. Higher Ag(+) concentrations favor a competitive thermal process, which results in increased prism thickness.
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Cites
Transmission Electron Microscopy of Shape-Controlled Nanocrystals and Their Assemblies
Wang, Z. L. (2000) · The Journal of Physical Chemistry B · doi:10.1021/jp993593c · Cited by 2,137
Photochemistry on Metal Nanoparticles
Watanabe, K., Menzel, D., Nilius, N., & Freund, H.-J. (2006) · Chemical Reviews · doi:10.1021/cr050167g · Cited by 486
Cited by
Colloidal Gold and Silver Triangular Nanoprisms
Millstone, J. E., Hurst, S. J., Métraux, G. S., Cutler, J. I., & Mirkin, C. A. (2009) · Small · doi:10.1002/smll.200801480 · Cited by 895
Self-citationMaking Sense of the Mayhem behind Shape Control in the Synthesis of Gold Nanoparticles
Personick, M. L., & Mirkin, C. A. (2013) · Journal of the American Chemical Society · doi:10.1021/ja408645b · Cited by 363
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Metadata
- Authors
- Xue, C., Métraux, G. S., Millstone, J. E., & Mirkin, C. A.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2008-06-06
- Volume
- 130
- Issue
- 26
- Pages
- 8337-8344
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W1972560232
- Cited by
- 413
- References
- 2
- FWCI
- 9.50
- Type
- journal article
- Language
- en
- Open access
- green
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- Xue, C., Métraux, G. S., Millstone, J. E., & Mirkin, C. A. (2008). Mechanistic Study of Photomediated Triangular Silver Nanoprism Growth. Journal of the American Chemical Society. https://doi.org/10.1021/ja8005258
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