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Mononuclear Lanthanide Single-Molecule Magnets Based on Polyoxometalates
Abstract
[ErW10O36]9- is the first polyoxometalate behaving as a single-molecule magnet (SMM). It shows frequency-dependent out-of-phase magnetization and a thermally activated single relaxation process with an effective barrier of 55.8 K. This single lanthanide ion polyoxometalate is the inorganic analogue of the bis(phthalocyaninato)lanthanide SMMs, both exhibiting very similar ligand field symmetries around the lanthanide ion (idealized D4d). It is chemically stable and offers new avenues for organization and processing of single-molecule magnets. Furthermore, it can be made free from nuclear spins and opens the possibility to be used for studies of decoherence on unimolecular qubits.
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Cites
Dispersion and Absorption in Dielectrics I. Alternating Current Characteristics
Cole, K. S., & Cole, R. H. (1941) · The Journal of Chemical Physics · doi:10.1063/1.1750906 · Cited by 10,152
Cited by
Lanthanide Single-Molecule Magnets
Woodruff, D. N., Winpenny, R. E. P., & Layfield, R. A. (2013) · Chemical Reviews · doi:10.1021/cr400018q · Cited by 2,781
Slow magnetization dynamics in a series of two-coordinate iron(ii) complexes
Zadrozny, J. M., Atanasov, M., Bryan, A. M., Lin, C.-Y., Rekken, B. D., Power, P. P., Neese, F., & Long, J. R. (2013) · Chem. Sci. · doi:10.1039/c2sc20801f · Cited by 579
Nielsen, V. R. M., & Just Sørensen, T. (2025) · Nature Communications · doi:10.1038/s41467-025-66054-7 · Cited by 5
Metadata
- Authors
- AlDamen, M. A., Clemente-Juan, J. M., Coronado, E., Martí-Gastaldo, C., & Gaita-Ariño, A.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2008-06-18
- Volume
- 130
- Issue
- 28
- Pages
- 8874-8875
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2070150426
- Cited by
- 863
- References
- 1
- FWCI
- 22.79
- Type
- journal article
- Language
- en
- Open access
- closed
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