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Liquid Phase Adsorption by Microporous Coordination Polymers: Removal of Organosulfur Compounds
Abstract
The utility of microporous coordination polymers (MCPs) for the adsorption of large organosulfur compounds (benzothiophene, dibenzothiophene, 4,6-dimethyldibenzothiophene) found in fuels is demonstrated. Large capacities are obtained at both low and high sulfur concentrations. For 4,6-dimethyldibenzothiophene, the compound most difficult to remove using current industrial techniques, a capacity of 41 g S/kg MCP at 1500 ppmw S is achieved by UMCM-150. It was determined that the size/shape of the pores in the MCP, rather than the surface area or pore volume, is the most important factor controlling adsorption capacity.
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Cited by
Metal–Organic Frameworks for Separations
Li, J.-R., Sculley, J., & Zhou, H.-C. (2012) · Chemical Reviews · doi:10.1021/cr200190s · Cited by 6,323
Adsorptive separation on metal–organic frameworks in the liquid phase
Van de Voorde, B., Bueken, B., Denayer, J., & De Vos, D. (2014) · Chem. Soc. Rev. · doi:10.1039/c4cs00006d · Cited by 874
Carné-Sánchez, A., Imaz, I., Cano-Sarabia, M., & Maspoch, D. (2013) · Nature Chemistry · doi:10.1038/nchem.1569 · Cited by 678
Zhu, X., Li, B., Yang, J., Li, Y., Zhao, W., Shi, J., & Gu, J. (2015) · ACS Applied Materials & Interfaces · doi:10.1021/am5059074 · Cited by 486
Adsorptive desulfurization and denitrogenation using metal-organic frameworks
Ahmed, I., & Jhung, S. H. (2016) · Journal of Hazardous Materials · doi:10.1016/j.jhazmat.2015.08.045 · Cited by 451
Metadata
- Authors
- Cychosz, K. A., Wong-Foy, A. G., & Matzger, A. J.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2008-05-09
- Volume
- 130
- Issue
- 22
- Pages
- 6938-6939
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2088362985
- Cited by
- 391
- References
- 0
- FWCI
- 46.94
- Type
- journal article
- Language
- en
- Open access
- closed
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- Cychosz, K. A., Wong-Foy, A. G., & Matzger, A. J. (2008). Liquid Phase Adsorption by Microporous Coordination Polymers: Removal of Organosulfur Compounds. Journal of the American Chemical Society. https://doi.org/10.1021/ja802121u
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