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Chirality-Controlled and Solvent-Templated Catenation Isomerism in Metal−Organic Frameworks
Abstract
A family of highly porous homochiral, racemic, and meso metal-organic frameworks (MOFs) were synthesized based on a new elongated tetra-carboxylate ligand and the copper paddle-wheel building units. These MOFs exhibited remarkable catenation isomerism that is controlled by both chirality of the bridging ligand and the size of solvent molecules. The ability to manipulate framework interpenetration is key to future synthesis of mesoporous homochiral MOFs which hold great promise in heterogeneous asymmetric catalysis and chiral separations.
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Citations
Cited by
Mesoporous metal–organic framework materials
Xuan, W., Zhu, C., Liu, Y., & Cui, Y. (2012) · Chem. Soc. Rev. · doi:10.1039/c1cs15196g · Cited by 933
Liu, Y., Xuan, W., & Cui, Y. (2010) · Advanced Materials · doi:10.1002/adma.201000197 · Cited by 872
Stepwise Synthesis of Metal–Organic Frameworks: Replacement of Structural Organic Linkers
Burnett, B. J., Barron, P. M., Hu, C., & Choe, W. (2011) · Journal of the American Chemical Society · doi:10.1021/ja201911v · Cited by 329
Activation of metal–organic framework materials
Mondloch, J. E., Karagiaridi, O., Farha, O. K., & Hupp, J. T. (2013) · CrystEngComm · doi:10.1039/c3ce41232f · Cited by 324
Deng, W., Fan, C., Zhang, R., & Jin, M. (2024) · Foods · doi:10.3390/foods13223614 · Cited by 31
Metadata
- Authors
- Ma, L., & Lin, W.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2008-09-30
- Volume
- 130
- Issue
- 42
- Pages
- 13834-13835
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2016531024
- Cited by
- 257
- References
- 0
- FWCI
- 17.61
- Type
- journal article
- Language
- en
- Open access
- closed
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- Ma, L., & Lin, W. (2008). Chirality-Controlled and Solvent-Templated Catenation Isomerism in Metal−Organic Frameworks. Journal of the American Chemical Society. https://doi.org/10.1021/ja804944r
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