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Probing the Structure of Single-Molecule Surface-Enhanced Raman Scattering Hot Spots
Abstract
We present here a detailed study of the specific nanoparticle structures that give rise to single-molecule surface-enhanced Raman scattering (SMSERS). A variety of structures are observed, but the simplest are dimers of Ag nanocrystals. We chose one of these structures for detailed study using electrodynamics calculations and found that the electromagnetic SERS enhancement factors of 10(9) are easily obtained and are consistent with single-molecule SERS activity.
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Citations
Cited by
Dasary, S. S. R., Singh, A. K., Senapati, D., Yu, H., & Ray, P. C. (2009) · Journal of the American Chemical Society · doi:10.1021/ja905134d · Cited by 722
Fundamental understanding and applications of plasmon-enhanced Raman spectroscopy
Wang, X., Huang, S.-C., Hu, S., Yan, S., & Ren, B. (2020) · Nature Reviews Physics · doi:10.1038/s42254-020-0171-y · Cited by 689
Guerrini, L., & Graham, D. (2012) · Chemical Society Reviews · doi:10.1039/c2cs35118h · Cited by 441
Molecular cavity optomechanics as a theory of plasmon-enhanced Raman scattering
Roelli, P., Galland, C., Piro, N., & Kippenberg, T. J. (2016) · Nature Nanotechnology · doi:10.1038/nnano.2015.264 · Cited by 276
Characterization of Nanomaterials
Mudalige, T., Qu, H., Van Haute, D., Ansar, S. M., Paredes, A., & Ingle, T. (2019) · Nanomaterials for Food Applications · doi:10.1016/b978-0-12-814130-4.00011-7 · Cited by 261
Metadata
- Authors
- Camden, J. P., Dieringer, J. A., Wang, Y., Masiello, D. J., Marks, L. D., Schatz, G. C., & Van Duyne, R. P.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2008-08-30
- Volume
- 130
- Issue
- 38
- Pages
- 12616-12617
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2064796543
- Cited by
- 943
- References
- 0
- FWCI
- 21.65
- Type
- journal article
- Language
- en
- Open access
- closed
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- Camden, J. P., Dieringer, J. A., Wang, Y., Masiello, D. J., Marks, L. D., Schatz, G. C., & Van Duyne, R. P. (2008). Probing the Structure of Single-Molecule Surface-Enhanced Raman Scattering Hot Spots. Journal of the American Chemical Society. https://doi.org/10.1021/ja8051427
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