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Activation of H2 by Phosphinoboranes R2PB(C6F5)2
Abstract
Phosphinoboranes that combine bulky electron-rich phosphides and electron deficient B(C6F5)2 fragments produce monomeric phosphinoboranes that undergo facile addition of H2 to give the phosphine-borane adducts (R2PH)(HBR'2). This finding in combination with DFT calculations shed light on the uptake of H2 across a group 13-group 15 bond, a critical requirement for the development of recyclable H2 storage materials.
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Cites
Ni1-xPtx (x = 0−0.12) Hollow Spheres as Catalysts for Hydrogen Generation from Ammonia Borane
Cheng, F., Ma, H., Li, Y., & Chen, J. (2007) · Inorganic Chemistry · doi:10.1021/ic061712e · Cited by 349
Cited by
Fischer, R. C., & Power, P. P. (2010) · Chemical Reviews · doi:10.1021/cr100133q · Cited by 1,155
B–N compounds for chemical hydrogenstorage
Hamilton, C. W., Baker, R. T., Staubitz, A., & Manners, I. (2009) · Chem. Soc. Rev. · doi:10.1039/b800312m · Cited by 1,087
Rokob, T. A., Hamza, A., & Pápai, I. (2009) · Journal of the American Chemical Society · doi:10.1021/ja903878z · Cited by 324
Enantioselective Hydrogenation with Chiral Frustrated Lewis Pairs
Chen, D., Wang, Y., & Klankermayer, J. (2010) · Angewandte Chemie International Edition · doi:10.1002/anie.201004525 · Cited by 295
Metadata
- Authors
- Geier, S. J., Gilbert, T. M., & Stephan, D. W.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2008-08-28
- Volume
- 130
- Issue
- 38
- Pages
- 12632-12633
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2330222529
- Cited by
- 187
- References
- 1
- FWCI
- 13.21
- Type
- journal article
- Language
- en
- Open access
- closed
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- Geier, S. J., Gilbert, T. M., & Stephan, D. W. (2008). Activation of H2 by Phosphinoboranes R2PB(C6F5)2. Journal of the American Chemical Society. https://doi.org/10.1021/ja805493y
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Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
