The DOI matches its Crossref record; 26 of the 26 references it cites were found in a registry or an index.
“Molecular Basket” Sorbents for Separation of CO2 and H2S from Various Gas Streams
Abstract
A new generation of "molecular basket" sorbents (MBS) has been developed by the optimum combination of the nanoporous material and CO(2)/H(2)S-philic polymer sorbent to increase the accessible sorption sites for CO(2) capture from flue gas (Postdecarbonization), and for CO(2) and H(2)S separation from the reduced gases, such as synthesis gas, reformate (Predecarbonization), natural gas, coal/biomass gasification gas, and biogas. The sorption capacity of 140 mg of CO(2)/g of sorb was achieved at 15 kPa CO(2) partial pressure, which shows superior performance in comparison with other known sorbents. In addition, an exceptional dependence of MBS sorption performance on temperature for CO(2) and H(2)S was found and discussed at a molecular level via the computational chemistry approach. On the basis of the fundamental understanding of MBS sorption characteristics, an innovative sorption process was proposed and demonstrated at the laboratory scale for removing and recovering CO(2) and H(2)S, respectively, from a model gas. The present study provides a new approach for development of the novel CO(2)/H(2)S sorbents and may have a major impact on the advance of science and technology for CO(2)/H(2)S capture and separation from various gases.
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Cited by
Post-Combustion CO 2 Capture Using Solid Sorbents: A Review
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A Review of CO2 Capture by Absorption and Adsorption
Yu, C.-H., Huang, C.-H., & Tan, C.-S. (2012) · Aerosol and Air Quality Research · doi:10.4209/aaqr.2012.05.0132 · Cited by 1,730
Adsorption of Carbon Dioxide for post-combustion capture: a review
Raganati, F., Miccio, F., & Ammendola, P. (2021) · Energy & Fuels · doi:10.1021/acs.energyfuels.1c01618 · Cited by 661
Understanding the Effect of Water on CO2 Adsorption
Kolle, J. M., Fayaz, M., & Sayari, A. (2021) · Chemical Reviews · doi:10.1021/acs.chemrev.0c00762 · Cited by 523
Carbon dioxide utilization with C–N bond formation: carbon dioxide capture and subsequent conversion
Yang, Z.-Z., He, L.-N., Gao, J., Liu, A.-H., & Yu, B. (2012) · Energy & Environmental Science · doi:10.1039/c2ee02774g · Cited by 520
Metadata
- Authors
- Ma, X., Wang, X., & Song, C.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2009-04-06
- Volume
- 131
- Issue
- 16
- Pages
- 5777-5783
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2008549335
- Cited by
- 532
- References
- 26
- FWCI
- 66.55
- Type
- journal article
- Language
- en
- Open access
- closed
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