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“Twin Copper Source” Growth of Metal−Organic Framework Membrane: Cu3(BTC)2 with High Permeability and Selectivity for Recycling H2
Abstract
In this communication, the copper net supported Cu(3)(BTC)(2) membranes have been successfully synthesized by means of a "twin copper source" technique. Separation studies on gaseous mixtures (H(2)/CO(2), H(2)/CH(4), and H(2)/N(2)) using the membrane revealed that the membrane possesses high permeability and selectivity for H(2) over CO(2), N(2), and CH(4). Compared with the conventional zeolite membranes, the copper net supported Cu(3)(BTC)(2) membrane exhibited high permeation flux in gas separation. Such highly efficient copper net supported Cu(3)(BTC)(2) membranes could be used to separate, recycle, and reuse H(2) exhausted from steam reforming natural gas.
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Citations
Cited by
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Li, J.-R., Sculley, J., & Zhou, H.-C. (2012) · Chemical Reviews · doi:10.1021/cr200190s · Cited by 6,323
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D'Alessandro, D. M., Smit, B., & Long, J. R. (2010) · Angewandte Chemie International Edition · doi:10.1002/anie.201000431 · Cited by 4,046
Zhan, W.-W., Kuang, Q., Zhou, J.-Z., Kong, X.-J., Xie, Z.-X., & Zheng, L.-S. (2013) · Journal of the American Chemical Society · doi:10.1021/ja311085e · Cited by 803
MOF positioning technology and device fabrication
Falcaro, P., Ricco, R., Doherty, C. M., Liang, K., Hill, A. J., & Styles, M. J. (2014) · Chem. Soc. Rev. · doi:10.1039/c4cs00089g · Cited by 710
Bae, T., Lee, J. S., Qiu, W., Koros, W. J., Jones, C. W., & Nair, S. (2010) · Angewandte Chemie International Edition · doi:10.1002/anie.201006141 · Cited by 678
Metadata
- Authors
- Guo, H., Zhu, G., Hewitt, I. J., & Qiu, S.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2009-01-21
- Volume
- 131
- Issue
- 5
- Pages
- 1646-1647
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2069202835
- Cited by
- 591
- References
- 0
- FWCI
- 98.50
- Type
- journal article
- Language
- en
- Open access
- closed
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- Guo, H., Zhu, G., Hewitt, I. J., & Qiu, S. (2009). “Twin Copper Source” Growth of Metal−Organic Framework Membrane: Cu3(BTC)2 with High Permeability and Selectivity for Recycling H2. Journal of the American Chemical Society. https://doi.org/10.1021/ja8074874
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