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Single-Site, Catalytic Water Oxidation on Oxide Surfaces
Abstract
Electrocatalytic water oxidation occurs through the use of the phosphonate-derivatized single-site catalyst [Ru(Mebimpy)(4,4'-((HO)(2)OPCH(2))(2)bpy)(OH(2))](2+) [Mebimpy = 2,6-bis(1-methylbenzimidazol-2-yl)pyridine; bpy = 2,2'-bipyridine] at pH 1 and 5 on fluorine-doped SnO(2) or Sn(IV)-doped In(2)O(3) electrodes or on nanocrystalline TiO(2). The surface-bound catalyst appears to retain the water oxidation mechanism found for [Ru(tpy)(bpm)(OH(2))](2+) and [Ru(tpy)(bpz)(OH(2))](2+) (tpy = 2,2':6',2''-terpyridine; bpm = 2,2'-bipyrimidine; bpz = 2,2'-bipyrazine) in solution and acts as a surface electrocatalyst for sustained water oxidation.
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Cited by
The Mechanism of Water Oxidation: From Electrolysis via Homogeneous to Biological Catalysis
Dau, H., Limberg, C., Reier, T., Risch, M., Roggan, S., & Strasser, P. (2010) · ChemCatChem · doi:10.1002/cctc.201000126 · Cited by 1,783
Metadata
- Authors
- Chen, Z., Concepcion, J. J., Jurss, J. W., & Meyer, T. J.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2009-10-09
- Volume
- 131
- Issue
- 43
- Pages
- 15580-15581
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W1967045707
- Cited by
- 245
- References
- 0
- FWCI
- 11.53
- Type
- journal article
- Language
- en
- Open access
- closed
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- Chen, Z., Concepcion, J. J., Jurss, J. W., & Meyer, T. J. (2009). Single-Site, Catalytic Water Oxidation on Oxide Surfaces. Journal of the American Chemical Society. https://doi.org/10.1021/ja906391w
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