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Hydrogen Storage by Boron−Nitrogen Heterocycles: A Simple Route for Spent Fuel Regeneration
Abstract
We describe a new hydrogen storage platform based on well-defined BN heterocyle materials. Specifically, we demonstrate that regeneration of the spent fuel back to the charged fuel can be accomplished using molecular H(2) and H(-)/H(+) sources. Crystallographic characterization of intermediates along the regeneration pathway confirms our structural assignments and reveals unique bonding changes associated with increasing hydrogen content on boron and nitrogen. Synthetic access to the fully charged BN cyclohexane fuels will now enable investigations of these materials in hydrogen desorption studies.
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Citations
Cites
B–N compounds for chemical hydrogenstorage
Hamilton, C. W., Baker, R. T., Staubitz, A., & Manners, I. (2009) · Chem. Soc. Rev. · doi:10.1039/b800312m · Cited by 1,087
Cited by
(2018) · doi:10.1016/j.enconman.2018.03.088 · Cited by 1,832
(2021) · doi:10.1016/j.rser.2021.111311 · Cited by 850
Liquid Organic Hydrogen Carrier (LOHC)—Assessment based on chemical and economic properties
Niermann, M., Beckendorff, A., Kaltschmitt, M., & Bonhoff, K. (2019) · International Journal of Hydrogen Energy · doi:10.1016/j.ijhydene.2019.01.199 · Cited by 635
BN Heterosuperbenzenes: Synthesis and Properties
Wang, X., Wang, J., & Pei, J. (2015) · Chemistry – A European Journal · doi:10.1002/chem.201405627 · Cited by 447
Hydrogen economy, energy, and liquid organic carriers for its mobility
Singh, R., Singh, M., & Gautam, S. (2021) · Materials Today: Proceedings · doi:10.1016/j.matpr.2020.09.065 · Cited by 148
Metadata
- Authors
- Campbell, P. G., Zakharov, L. N., Grant, D. J., Dixon, D. A., & Liu, S.-Y.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2010-02-19
- Volume
- 132
- Issue
- 10
- Pages
- 3289-3291
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W1989873887
- Cited by
- 168
- References
- 1
- FWCI
- 7.72
- Type
- journal article
- Language
- en
- Open access
- closed
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- Campbell, P. G., Zakharov, L. N., Grant, D. J., Dixon, D. A., & Liu, S.-Y. (2010). Hydrogen Storage by Boron−Nitrogen Heterocycles: A Simple Route for Spent Fuel Regeneration. Journal of the American Chemical Society. https://doi.org/10.1021/ja9106622
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
