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Catalytic Oxidation of Carbon Monoxide on Monodispersed Platinum Clusters: Each Atom Counts
Open accessAbstract
Nanoclusters open fascinating opportunities for quantum engineering because quantum-size effects become dominant in determining catalytic, 1 - 3 optical, 4 electronic, 5 and magnetic 6 properties. We succeeded in the controlled production of low-energy and high-flux monodispersed cluster beams, which allow for a systematic study of their reactivity after deposition onto a chemically inert substrate. We investigated the catalytic reaction that is the oxidation of CO on platinum and observed a distinct atom by atom size dependency for monodispersed platinum clusters on thin MgO(100) films. These results clearly show that the efficiency of a heterogeneous catalytic reaction can be tuned by the judicious choice of particle size.
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Cites
Effect of seawater carbonate concentration on foraminiferal carbon and oxygen isotopes
Spero, H. J., Bijma, J., Lea, D. W., & Bemis, B. E. (1997) · Nature · doi:10.1038/37333 · Cited by 975
Cited by
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New trends in tailoring active sites in zeolite-based catalysts
Shamzhy, M., Opanasenko, M., Concepción, P., & Martínez, A. (2019) · Chemical Society Reviews · doi:10.1039/c8cs00887f · Cited by 508
Liu, M., Wang, L., Zhao, K., Shi, S., Shao, Q., Zhang, L., Sun, X., Zhao, Y., & Zhang, J. (2019) · Energy & Environmental Science · doi:10.1039/c9ee01722d · Cited by 429
Synthetic strategies of supported atomic clusters for heterogeneous catalysis
Rong, H., Ji, S., Zhang, J., Wang, D., & Li, Y. (2020) · Nature Communications · doi:10.1038/s41467-020-19571-6 · Cited by 367
The Power of Single‐Atom Catalysis
Liang, S., Hao, C., & Shi, Y. (2015) · ChemCatChem · doi:10.1002/cctc.201500363 · Cited by 365
Metadata
- Authors
- Heiz, U., Sanchez, A., Abbet, S., & Schneider, W.-D.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 1999-03-19
- Volume
- 121
- Issue
- 13
- Pages
- 3214-3217
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2044768445
- Cited by
- 505
- References
- 1
- FWCI
- 12.87
- Type
- journal article
- Language
- en
- Open access
- green
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