The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Core−Shell Gyroid Morphology in a Poly(isoprene-block-styrene-block-dimethylsiloxane) Triblock Copolymer
Abstract
We report a new morphology in a poly(isoprene- block -styrene- block -dimethylsiloxane) ABC triblock copolymer. The most probable symmetry of the morphology ( Ia 3̄ d ) was determined from two-dimensional SAXS measurements performed on a sample with long-range order induced by an oscillatory shear field. By comparing the predictions of self-consistent field theory with TEM and SAXS and SANS powder diffraction patterns, we deduced that the morphology is a core−shell gyroid comprised of two independent and triply periodic poly(dimethylsiloxane) networks encased in poly(styrene) shells and separated by a continuous poly(isoprene) domain. Thus, this unique nanostructure divides space into five independent, three-dimensionally continuous domains.
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Cites
Fetters, L. J., Lohse, D. J., Richter, D., Witten, T. A., & Zirkel, A. (1994) · Macromolecules · doi:10.1021/ma00095a001 · Cited by 1,999
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Self-citationHan, L., & Che, S. (2018) · Advanced Materials · doi:10.1002/adma.201705708 · Cited by 624
HADJICHRISTIDIS, N., IATROU, H., PITSIKALIS, M., PISPAS, S., & AVGEROPOULOS, A. (2005) · Progress in Polymer Science · doi:10.1016/j.progpolymsci.2005.04.001 · Cited by 428
Thermoplastic elastomers: fundamentals and applications
Spontak, R. J., & Patel, N. P. (2000) · Current Opinion in Colloid & Interface Science · doi:10.1016/s1359-0294(00)00070-4 · Cited by 408
Phase Behaviour and Morphologies of Block Copolymers
Abetz, V., & Simon, P. F. W. (2005) · Advances in Polymer Science · doi:10.1007/12_004 · Cited by 361
Metadata
- Authors
- Shefelbine, T. A., Vigild, M. E., Matsen, M. W., Hajduk, D. A., Hillmyer, M. A., Cussler, E. L., & Bates, F. S.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 1999-09-01
- Volume
- 121
- Issue
- 37
- Pages
- 8457-8465
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W1984574554
- Cited by
- 207
- References
- 1
- FWCI
- 7.15
- Type
- journal article
- Language
- en
- Open access
- closed
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
