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Highly Water-Stable Zirconium Metal–Organic Framework UiO-66 Membranes Supported on Alumina Hollow Fibers for Desalination
Open accessAbstract
In this study, continuous zirconium(IV)-based metal-organic framework (Zr-MOF) membranes were prepared. The pure-phase Zr-MOF (i.e., UiO-66) polycrystalline membranes were fabricated on alumina hollow fibers using an in situ solvothermal synthesis method. Single-gas permeation and ion rejection tests were carried out to confirm membrane integrity and functionality. The membrane exhibited excellent multivalent ion rejection (e.g., 86.3% for Ca(2+), 98.0% for Mg(2+), and 99.3% for Al(3+)) on the basis of size exclusion with moderate permeance (0.14 L m(-2) h(-1) bar(-1)) and good permeability (0.28 L m(-2) h(-1) bar(-1) μm). Benefiting from the exceptional chemical stability of the UiO-66 material, no degradation of membrane performance was observed for various tests up to 170 h toward a wide range of saline solutions. The high separation performance combined with its outstanding water stability suggests the developed UiO-66 membrane as a promising candidate for water desalination.
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Cites
Phenomenological Theory of Ion Solvation. Effective Radii of Hydrated Ions
Nightingale, E. R. (1959) · The Journal of Physical Chemistry · doi:10.1021/j150579a011 · Cited by 3,505
Cited by
Yusuf, V. F., Malek, N. I., & Kailasa, S. K. (2022) · ACS Omega · doi:10.1021/acsomega.2c05310 · Cited by 894
Metal–organic frameworks for membrane-based separations
Denny, M. S., Moreton, J. C., Benz, L., & Cohen, S. M. (2016) · Nature Reviews Materials · doi:10.1038/natrevmats.2016.78 · Cited by 820
Fan, H., Gu, J., Meng, H., Knebel, A., & Caro, J. (2018) · Angewandte Chemie International Edition · doi:10.1002/anie.201712816 · Cited by 804
Advanced Porous Materials in Mixed Matrix Membranes
Cheng, Y., Ying, Y., Japip, S., Jiang, S., Chung, T., Zhang, S., & Zhao, D. (2018) · Advanced Materials · doi:10.1002/adma.201802401 · Cited by 448
Advances in metal–organic framework-based membranes
Cheng, Y., Datta, S. J., Zhou, S., Jia, J., Shekhah, O., & Eddaoudi, M. (2022) · Chemical Society Reviews · doi:10.1039/d2cs00031h · Cited by 423
Metadata
- Authors
- Liu, X., Demir, N. K., Wu, Z., & Li, K.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-06-01
- Volume
- 137
- Issue
- 22
- Pages
- 6999-7002
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2410849299
- Cited by
- 802
- References
- 1
- FWCI
- 35.87
- Type
- journal article
- Language
- en
- Open access
- green
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- Liu, X., Demir, N. K., Wu, Z., & Li, K. (2015). Highly Water-Stable Zirconium Metal–Organic Framework UiO-66 Membranes Supported on Alumina Hollow Fibers for Desalination. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.5b02276
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