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Carbon Dioxide Conversion to Methanol over Size-Selected Cu4 Clusters at Low Pressures
Open accessAbstract
The activation of CO2 and its hydrogenation to methanol are of much interest as a way to utilize captured CO2. Here, we investigate the use of size-selected Cu4 clusters supported on Al2O3 thin films for CO2 reduction in the presence of hydrogen. The catalytic activity was measured under near-atmospheric reaction conditions with a low CO2 partial pressure, and the oxidation state of the clusters was investigated by in situ grazing incidence X-ray absorption spectroscopy. The results indicate that size-selected Cu4 clusters are the most active low-pressure catalyst for catalytic CO2 conversion to CH3OH. Density functional theory calculations reveal that Cu4 clusters have a low activation barrier for conversion of CO2 to CH3OH. This study suggests that small Cu clusters may be excellent and efficient catalysts for the recycling of released CO2.
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Fe and Pt carbon nanotubes for the electrocatalytic conversion of carbon dioxide to oxygenates
Gangeri, M., Perathoner, S., Caudo, S., Centi, G., Amadou, J., Bégin, D., Pham-Huu, C., Ledoux, M. J., Tessonnier, J.-P., & Su, D. S. (2009) · Catalysis Today · doi:10.1016/j.cattod.2008.11.001 · Cited by 112
Cited by
Tuning Selectivity of CO2 Hydrogenation Reactions at the Metal/Oxide Interface
Kattel, S., Liu, P., & Chen, J. G. (2017) · Journal of the American Chemical Society · doi:10.1021/jacs.7b05362 · Cited by 1,259
Wu, J., Ma, S., Sun, J., Gold, J. I., Tiwary, C., Kim, B., Zhu, L., Chopra, N., Odeh, I. N., Vajtai, R., et al. (2016) · Nature Communications · doi:10.1038/ncomms13869 · Cited by 658
Rungtaweevoranit, B., Baek, J., Araujo, J. R., Archanjo, B. S., Choi, K. M., Yaghi, O. M., & Somorjai, G. A. (2016) · Nano Letters · doi:10.1021/acs.nanolett.6b03637 · Cited by 459
Significant Advances in C1 Catalysis: Highly Efficient Catalysts and Catalytic Reactions
Bao, J., Yang, G., Yoneyama, Y., & Tsubaki, N. (2019) · ACS Catalysis · doi:10.1021/acscatal.8b03924 · Cited by 367
Catalysis Applications of Size-Selected Cluster Deposition
Vajda, S., & White, M. G. (2015) · ACS Catalysis · doi:10.1021/acscatal.5b01816 · Cited by 293
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Metadata
- Authors
- Liu, C., Yang, B., Tyo, E., Seifert, S., DeBartolo, J., von Issendorff, B., Zapol, P., Vajda, S., & Curtiss, L. A.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-07-02
- Volume
- 137
- Issue
- 27
- Pages
- 8676-8679
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W1001544694
- Cited by
- 389
- References
- 1
- FWCI
- 10.63
- Type
- journal article
- Language
- en
- Open access
- green
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- Liu, C., Yang, B., Tyo, E., Seifert, S., DeBartolo, J., von Issendorff, B., Zapol, P., Vajda, S., & Curtiss, L. A. (2015). Carbon Dioxide Conversion to Methanol over Size-Selected Cu4 Clusters at Low Pressures. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.5b03668
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