The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
Synthesis and Characterization of Iron–Nitrogen-Doped Graphene/Core–Shell Catalysts: Efficient Oxidative Dehydrogenation of N-Heterocycles
Abstract
An important goal for nanocatalysis is the development of flexible and efficient methods for preparing active and stable core-shell catalysts. In this respect, we present the synthesis and characterization of iron oxides surrounded by nitrogen-doped-graphene shells immobilized on carbon support (labeled FeOx@NGr-C). Active catalytic materials are obtained in a simple, scalable and two-step method via pyrolysis of iron acetate and phenanthroline and subsequent selective leaching. The optimized FeOx@NGr-C catalyst showed high activity in oxidative dehydrogenations of several N-heterocycles. The utility of this benign methodology is demonstrated by the synthesis of pharmaceutically relevant quinolines. In addition, mechanistic studies prove that the reaction progresses via superoxide radical anions (·O2(-)).
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Cites
High-Performance Electrocatalysts for Oxygen Reduction Derived from Polyaniline, Iron, and Cobalt
Wu, G., More, K. L., Johnston, C. M., & Zelenay, P. (2011) · Science · doi:10.1126/science.1200832 · Cited by 3,984
Zhang, S., Hao, Y., Su, D., Doan-Nguyen, V. V. T., Wu, Y., Li, J., Sun, S., & Murray, C. B. (2014) · Journal of the American Chemical Society · doi:10.1021/ja5099066 · Cited by 179
Cited by
He, L., Weniger, F., Neumann, H., & Beller, M. (2016) · Angewandte Chemie International Edition · doi:10.1002/anie.201603198 · Cited by 618
Self-citationThe recent development of efficient Earth-abundant transition-metal nanocatalysts
Wang, D., & Astruc, D. (2017) · Chemical Society Reviews · doi:10.1039/c6cs00629a · Cited by 608
Progress in the Chemistry of Tetrahydroquinolines
Muthukrishnan, I., Sridharan, V., & Menéndez, J. C. (2019) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00567 · Cited by 506
Yao, Y., Chen, H., Qin, J., Wu, G., Lian, C., Zhang, J., & Wang, S. (2016) · Water Research · doi:10.1016/j.watres.2016.05.065 · Cited by 332
Song, Y., Peng, R., Hensley, D. K., Bonnesen, P. V., Liang, L., Wu, Z., Meyer, H. M., Chi, M., Ma, C., Sumpter, B. G., et al. (2016) · ChemistrySelect · doi:10.1002/slct.201601169 · Cited by 328
Metadata
- Authors
- Cui, X., Li, Y., Bachmann, S., Scalone, M., Surkus, A.-E., Junge, K., Topf, C., & Beller, M.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-08-11
- Volume
- 137
- Issue
- 33
- Pages
- 10652-10658
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W968999674
- Cited by
- 299
- References
- 2
- FWCI
- 12.42
- Type
- journal article
- Language
- en
- Open access
- closed
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- Cui, X., Li, Y., Bachmann, S., Scalone, M., Surkus, A.-E., Junge, K., Topf, C., & Beller, M. (2015). Synthesis and Characterization of Iron–Nitrogen-Doped Graphene/Core–Shell Catalysts: Efficient Oxidative Dehydrogenation of N-Heterocycles. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.5b05674
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