The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
Electrochemical Tip-Enhanced Raman Spectroscopy
Abstract
Interfacial properties are highly important to the performance of some energy-related systems. The in-depth understanding of the interface requires highly sensitive in situ techniques that can provide fingerprint molecular information at nanometer resolution. We developed an electrochemical tip-enhanced Raman spectroscopy (EC-TERS) by introduction of the light horizontally to the EC-STM cell to minimize the optical distortion and to keep the TERS measurement under a well-controlled condition. We obtained potential-dependent EC-TERS from the adsorbed aromatic molecule on a Au(111) surface and observed a substantial change in the molecule configuration with potential as a result of the protonation and deprotonation of the molecule. Such a change was not observable in EC-SERS (surface-enhanced), indicating EC-TERS can more faithfully reflect the fine interfacial structure than EC-SERS. This work will open a new era for using EC-TERS as an important nanospectroscopy tool for the molecular level and nanoscale analysis of some important electrochemical systems including solar cells, lithium ion batteries, fuel cells, and corrosion.
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Cites
Raman spectra of pyridine adsorbed at a silver electrode
Fleischmann, M., Hendra, P. J., & McQuillan, A. J. (1974) · Chemical Physics Letters · doi:10.1016/0009-2614(74)85388-1 · Cited by 7,172
Surface raman spectroelectrochemistry
Jeanmaire, D. L., & Van Duyne, R. P. (1977) · Journal of Electroanalytical Chemistry and Interfacial Electrochemistry · doi:10.1016/s0022-0728(77)80224-6 · Cited by 4,738
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Fundamental understanding and applications of plasmon-enhanced Raman spectroscopy
Wang, X., Huang, S.-C., Hu, S., Yan, S., & Ren, B. (2020) · Nature Reviews Physics · doi:10.1038/s42254-020-0171-y · Cited by 689
Self-citationInfrared and Raman chemical imaging and spectroscopy at the nanoscale
Kurouski, D., Dazzi, A., Zenobi, R., & Centrone, A. (2020) · Chemical Society Reviews · doi:10.1039/c8cs00916c · Cited by 324
Chen, Z., Jiang, S., Kang, G., Nguyen, D., Schatz, G. C., & Van Duyne, R. P. (2019) · Journal of the American Chemical Society · doi:10.1021/jacs.9b07979 · Cited by 171
Influencing electrocatalytic processes through topographically disordered atomic sites
Prabhu, P., & Lee, J.-M. (2023) · Chem Catalysis · doi:10.1016/j.checat.2023.100621 · Cited by 84
Metadata
- Authors
- Zeng, Z.-C., Huang, S.-C., Wu, D.-Y., Meng, L.-Y., Li, M.-H., Huang, T.-X., Zhong, J.-H., Wang, X., Yang, Z.-L., & Ren, B.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-09-11
- Volume
- 137
- Issue
- 37
- Pages
- 11928-11931
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W1450920268
- Cited by
- 289
- References
- 2
- FWCI
- 10.41
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zeng, Z.-C., Huang, S.-C., Wu, D.-Y., Meng, L.-Y., Li, M.-H., Huang, T.-X., Zhong, J.-H., Wang, X., Yang, Z.-L., & Ren, B. (2015). Electrochemical Tip-Enhanced Raman Spectroscopy. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.5b08143
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