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Pt/In2S3/CdS/Cu2ZnSnS4 Thin Film as an Efficient and Stable Photocathode for Water Reduction under Sunlight Radiation
Abstract
An electrodeposited Cu2ZnSnS4 (CZTS) compact thin film modified with an In2S3/CdS double layer and Pt deposits (Pt/In2S3/CdS/CZTS) was used as a photocathode for water splitting of hydrogen production under simulated sunlight (AM 1.5G) radiation. Compared to platinized electrodes based on a bare CZTS film (Pt/CZTS) and a CZTS film modified with a CdS single layer (Pt/CdS/CZTS), the Pt/In2S3/CdS/CZTS electrode exhibited a significantly high cathodic photocurrent. Moreover, the coverage of the In2S3 layer was found to be effective for stabilization against degradation induced by photocorrosion of the CdS layer. Bias-free water splitting with a power conversion efficiency of 0.28% was achieved by using a simple two-electrode cell consisting of the Pt/In2S3/CdS/CZTS photocathode and a BiVO4 photoanode.
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Citations
Cites
Semiconductor-based Photocatalytic Hydrogen Generation
Chen, X., Shen, S., Guo, L., & Mao, S. S. (2010) · Chemical Reviews · doi:10.1021/cr1001645 · Cited by 7,876
Cited by
Yang, W., Prabhakar, R. R., Tan, J., Tilley, S. D., & Moon, J. (2019) · Chemical Society Reviews · doi:10.1039/c8cs00997j · Cited by 787
Recent Advances and Emerging Trends in Photo‐Electrochemical Solar Energy Conversion
Tilley, S. D. (2019) · Advanced Energy Materials · doi:10.1002/aenm.201802877 · Cited by 319
A Hollow Porous CdS Photocatalyst
Sun, Q., Wang, N., Yu, J., & Yu, J. C. (2018) · Advanced Materials · doi:10.1002/adma.201804368 · Cited by 293
Metadata
- Authors
- Jiang, F., Gunawan, Harada, T., Kuang, Y., Minegishi, T., Domen, K., & Ikeda, S.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-10-19
- Volume
- 137
- Issue
- 42
- Pages
- 13691-13697
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2283049464
- Cited by
- 289
- References
- 1
- FWCI
- 11.73
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: Pt/In2S3/CdS/Cu2ZnSnS4 Thin Film as an Efficient and Stable Photocathode for Water Reduction under Sunlight Radiation. https://app.cochat.ai/papers/10.1021/jacs.5b09015
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- Jiang, F., Gunawan, Harada, T., Kuang, Y., Minegishi, T., Domen, K., & Ikeda, S. (2015). Pt/In2S3/CdS/Cu2ZnSnS4 Thin Film as an Efficient and Stable Photocathode for Water Reduction under Sunlight Radiation. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.5b09015
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