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Photocatalytic CO2 Reduction Using Cu(I) Photosensitizers with a Fe(II) Catalyst
Open accessAbstract
Photocatalytic systems developed from complexes with only abundant metals, i.e., Cu(I)(dmp)(P)2(+) (dmp =2,9-dimethyl-1,10-phenanthroline; P = phosphine ligand) as a redox photosensitizer and Fe(II)(dmp)2(NCS)2 as a catalyst, produced CO as the main product by visible light irradiation. The best photocatalysis was obtained using a Cu(I) complex with a tetradentate dmp ligand tethering two phosphine groups, where the turnover number and quantum yield of CO formation were 273 and 6.7%, respectively.
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Cited by
Ong, W.-J., Tan, L.-L., Ng, Y. H., Yong, S.-T., & Chai, S.-P. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00075 · Cited by 7,147
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Dalle, K. E., Warnan, J., Leung, J. J., Reuillard, B., Karmel, I. S., & Reisner, E. (2019) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00392 · Cited by 912
Molecular polypyridine-based metal complexes as catalysts for the reduction of CO2
Elgrishi, N., Chambers, M. B., Wang, X., & Fontecave, M. (2017) · Chemical Society Reviews · doi:10.1039/c5cs00391a · Cited by 555
Boutin, E., Merakeb, L., Ma, B., Boudy, B., Wang, M., Bonin, J., Anxolabéhère-Mallart, E., & Robert, M. (2020) · Chemical Society Reviews · doi:10.1039/d0cs00218f · Cited by 423
Reaction mechanisms of catalytic photochemical CO2 reduction using Re(I) and Ru(II) complexes
Kuramochi, Y., Ishitani, O., & Ishida, H. (2018) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2017.11.023 · Cited by 325
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Metadata
- Authors
- Takeda, H., Ohashi, K., Sekine, A., & Ishitani, O.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-03-28
- Volume
- 138
- Issue
- 13
- Pages
- 4354-4357
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2306631785
- Cited by
- 321
- References
- 0
- FWCI
- 11.80
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- Takeda, H., Ohashi, K., Sekine, A., & Ishitani, O. (2016). Photocatalytic CO2 Reduction Using Cu(I) Photosensitizers with a Fe(II) Catalyst. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.6b01970
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